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Synthesis of Two-Dimensional CoS1.097/Nitrogen-Doped Carbon Nanocomposites Using Metal–Organic Framework Nanosheets as Precursors for Supercapacitor Application
Open accessAbstract
Two-dimensional (2D) metal-organic framework (MOF) nanosheets are attracting increasing research interest. Here, for the first time, we report the facile synthesis of 2D porphyrin paddlewheel framework-3 (PPF-3) MOF nanosheets with thickness of ca. 12-43 nm. Through the simultaneous sulfidation and carbonization of PPF-3 MOF nanosheets, we have prepared the 2D nanocomposite of CoS1.097 nanoparticles (NPs) and nitrogen-doped carbon, referred to as CoSNC, in which the CoS1.097 NPs with size of ca. 10 nm are embedded in the nitrogen-doped carbon matrix. As a proof-of-concept application, the obtained 2D CoSNC nanocomposite is used as an electrode material for a supercapacitor, which exhibits a specific capacitance of 360.1 F g(-1) at a current density of 1.5 A g(-1). Moreover, the composite electrode also shows high rate capability. Its specific capacitance delivered at a current density of 30.0 A g(-1) retains 56.8% of the value at 1.5 A g(-1).
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Cites
The chemistry of graphene oxide
Dreyer, D. R., Park, S., Bielawski, C. W., & Ruoff, R. S. (2010) · Chem. Soc. Rev. · doi:10.1039/b917103g · Cited by 11,653
You, B., Jiang, N., Sheng, M., Gul, S., Yano, J., & Sun, Y. (2015) · Chemistry of Materials · doi:10.1021/acs.chemmater.5b02877 · Cited by 631
Cited by
Wang, C., Kaneti, Y. V., Bando, Y., Lin, J., Liu, C., Li, J., & Yamauchi, Y. (2018) · Materials Horizons · doi:10.1039/c8mh00133b · Cited by 533
Zhou, S., Kong, X., Zheng, B., Huo, F., Strømme, M., & Xu, C. (2019) · ACS Nano · doi:10.1021/acsnano.9b04670 · Cited by 341
Rapid mass production of two-dimensional metal oxides and hydroxides via the molten salts method
Hu, Z., Xiao, X., Jin, H., Li, T., Chen, M., Liang, Z., Guo, Z., Li, J., Wan, J., Huang, L., et al. (2017) · Nature Communications · doi:10.1038/ncomms15630 · Cited by 328
Yang, N., Zhang, Z., Chen, B., Huang, Y., Chen, J., Lai, Z., Chen, Y., Sindoro, M., Wang, A., Cheng, H., et al. (2017) · Advanced Materials · doi:10.1002/adma.201700769 · Cited by 292
Self-citationEngineering 2D Architectures toward High‐Performance Micro‐Supercapacitors
Da, Y., Liu, J., Zhou, L., Zhu, X., Chen, X., & Fu, L. (2019) · Advanced Materials · doi:10.1002/adma.201802793 · Cited by 253
Metadata
- Authors
- Cao, F., Zhao, M., Yu, Y., Chen, B., Huang, Y., Yang, J., Cao, X., Lu, Q., Zhang, X., Zhang, Z., Tan, C., & Zhang, H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-05-24
- Volume
- 138
- Issue
- 22
- Pages
- 6924-6927
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2404600454
- Cited by
- 671
- References
- 2
- FWCI
- 32.35
- Type
- journal article
- Language
- en
- Open access
- green
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- The paper
- Cao, F., Zhao, M., Yu, Y., Chen, B., Huang, Y., Yang, J., Cao, X., Lu, Q., Zhang, X., Zhang, Z., Tan, C., & Zhang, H. (2016). Synthesis of Two-Dimensional CoS1.097/Nitrogen-Doped Carbon Nanocomposites Using Metal–Organic Framework Nanosheets as Precursors for Supercapacitor Application. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b02540
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