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Colloidal Synthesis of Quantum Confined Single Crystal CsPbBr3 Nanosheets with Lateral Size Control up to the Micrometer Range
Open accessAbstract
We report the nontemplated colloidal synthesis of single crystal CsPbBr3 perovskite nanosheets with lateral sizes up to a few micrometers and with thickness of just a few unit cells (i.e., below 5 nm), hence in the strong quantum confinement regime, by introducing short ligands (octanoic acid and octylamine) in the synthesis together with longer ones (oleic acid and oleylamine). The lateral size is tunable by varying the ratio of shorter ligands over longer ligands, while the thickness is mainly unaffected by this parameter and stays practically constant at 3 nm in all the syntheses conducted at short-to-long ligands volumetric ratio below 0.67. Beyond this ratio, control over the thickness is lost and a multimodal thickness distribution is observed.
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Cites
Graphene: Status and Prospects
Geim, A. K. (2009) · Science · doi:10.1126/science.1158877 · Cited by 13,942
Akkerman, Q. A., D’Innocenzo, V., Accornero, S., Scarpellini, A., Petrozza, A., Prato, M., & Manna, L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b05602 · Cited by 2,197
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Cited by
Zou, S., Liu, Y., Li, J., Liu, C., Feng, R., Jiang, F., Li, Y., Song, J., Zeng, H., Hong, M., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b04000 · Cited by 854
Recent advance in MXenes: A promising 2D material for catalysis, sensor and chemical adsorption
Zhu, J., Ha, E., Zhao, G., Zhou, Y., Huang, D., Yue, G., Hu, L., Sun, N., Wang, Y., Lee, L. Y. S., et al. (2017) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.09.012 · Cited by 659
Two-dimensional halide perovskite nanomaterials and heterostructures
Shi, E., Gao, Y., Finkenauer, B. P., Akriti, A., Coffey, A. H., & Dou, L. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00886d · Cited by 445
Perovskite semiconductors for room-temperature exciton-polaritonics
Su, R., Fieramosca, A., Zhang, Q., Nguyen, H. S., Deleporte, E., Chen, Z., Sanvitto, D., Liew, T. C. H., & Xiong, Q. (2021) · Nature Materials · doi:10.1038/s41563-021-01035-x · Cited by 255
Halide Ion Migration in Perovskite Nanocrystals and Nanostructures
Kamat, P. V., & Kuno, M. (2021) · Accounts of Chemical Research · doi:10.1021/acs.accounts.0c00749 · Cited by 219
Metadata
- Authors
- Shamsi, J., Dang, Z., Bianchini, P., Canale, C., Di Stasio, F., Brescia, R., Prato, M., & Manna, L.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-06-06
- Volume
- 138
- Issue
- 23
- Pages
- 7240-7243
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2400081589
- Cited by
- 503
- References
- 2
- FWCI
- 35.22
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Shamsi, J., Dang, Z., Bianchini, P., Canale, C., Di Stasio, F., Brescia, R., Prato, M., & Manna, L. (2016). Colloidal Synthesis of Quantum Confined Single Crystal CsPbBr3 Nanosheets with Lateral Size Control up to the Micrometer Range. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b03166
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