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Fabrication of COF-MOF Composite Membranes and Their Highly Selective Separation of H2/CO2
Abstract
The search for new types of membrane materials has been of continuous interest in both academia and industry, given their importance in a plethora of applications, particularly for energy-efficient separation technology. In this contribution, we demonstrate for the first time that a metal-organic framework (MOF) can be grown on the covalent-organic framework (COF) membrane to fabricate COF-MOF composite membranes. The resultant COF-MOF composite membranes demonstrate higher separation selectivity of H2/CO2 gas mixtures than the individual COF and MOF membranes. A sound proof for the synergy between two porous materials is the fact that the COF-MOF composite membranes surpass the Robeson upper bound of polymer membranes for mixture separation of a H2/CO2 gas pair and are among the best gas separation MOF membranes reported thus far.
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Citations
Cited by
Fan, H., Gu, J., Meng, H., Knebel, A., & Caro, J. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201712816 · Cited by 804
Wang, H., Zeng, Z., Xu, P., Li, L., Zeng, G., Xiao, R., Tang, Z., Huang, D., Tang, L., Lai, C., et al. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00376a · Cited by 804
Beuerle, F., & Gole, B. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201710190 · Cited by 528
Interfacial Polymerization: From Chemistry to Functional Materials
Zhang, F., Fan, J., & Wang, S. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201916473 · Cited by 478
Chiral covalent organic frameworks: design, synthesis and property
Han, X., Yuan, C., Hou, B., Liu, L., Li, H., Liu, Y., & Cui, Y. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00009d · Cited by 478
Metadata
- Authors
- Fu, J., Das, S., Xing, G., Ben, T., Valtchev, V., & Qiu, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-06-13
- Volume
- 138
- Issue
- 24
- Pages
- 7673-7680
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2403076599
- Cited by
- 614
- References
- 0
- FWCI
- 42.20
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fu, J., Das, S., Xing, G., Ben, T., Valtchev, V., & Qiu, S. (2016). Fabrication of COF-MOF Composite Membranes and Their Highly Selective Separation of H2/CO2. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b03348
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