The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Selective Gold Recovery and Catalysis in a Highly Flexible Methionine-Decorated Metal–Organic Framework
Open accessAbstract
A novel chiral 3D bioMOF exhibiting functional channels with thio-alkyl chains derived from the natural amino acid l-methionine (1) has been rationally prepared. The well-known strong affinity of gold for sulfur derivatives, together with the extremely high flexibility of the thioether "arms" decorating the channels, account for a selective capture of gold(III) and gold(I) salts in the presence of other metal cations typically found in electronic wastes. The X-ray single-crystal structures of the different gold adsorbates Au(III)@1 and Au(I)@1 suggest that the selective metal capture occurs in a metal ion recognition process somehow mimicking what happens in biological systems and protein receptors. Both Au(III)@1 and Au(I)@1 display high activity as heterogeneous catalyst for the hydroalkoxylation of alkynes, further expanding the application of these novel hybrid materials.
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Cites
BioMOFs: Metal–Organic Frameworks for Biological and Medical Applications
McKinlay, A. C., Morris, R. E., Horcajada, P., Férey, G., Gref, R., Couvreur, P., & Serre, C. (2010) · Angewandte Chemie International Edition · doi:10.1002/anie.201000048 · Cited by 1,256
Cited by
Metal–Organic Framework-Based Catalysts with Single Metal Sites
Wei, Y.-S., Zhang, M., Zou, R., & Xu, Q. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00757 · Cited by 1,233
A versatile MOF-based trap for heavy metal ion capture and dispersion
Peng, Y., Huang, H., Zhang, Y., Kang, C., Chen, S., Song, L., Liu, D., & Zhong, C. (2018) · Nature Communications · doi:10.1038/s41467-017-02600-2 · Cited by 804
Biological metal–organic frameworks: Structures, host–guest chemistry and bio-applications
Cai, H., Huang, Y.-L., & Li, D. (2019) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.12.003 · Cited by 419
Sun, D. T., Gasilova, N., Yang, S., Oveisi, E., & Queen, W. L. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b09555 · Cited by 366
Fortea-Pérez, F. R., Mon, M., Ferrando-Soria, J., Boronat, M., Leyva-Pérez, A., Corma, A., Herrera, J. M., Osadchii, D., Gascon, J., Armentano, D., et al. (2017) · Nature Materials · doi:10.1038/nmat4910 · Cited by 287
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Metadata
- Authors
- Mon, M., Ferrando-Soria, J., Grancha, T., Fortea-Pérez, F. R., Gascon, J., Leyva-Pérez, A., Armentano, D., & Pardo, E.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-06-16
- Volume
- 138
- Issue
- 25
- Pages
- 7864-7867
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2442546023
- Cited by
- 274
- References
- 1
- FWCI
- 8.76
- Type
- journal article
- Language
- en
- Open access
- green
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- Mon, M., Ferrando-Soria, J., Grancha, T., Fortea-Pérez, F. R., Gascon, J., Leyva-Pérez, A., Armentano, D., & Pardo, E. (2016). Selective Gold Recovery and Catalysis in a Highly Flexible Methionine-Decorated Metal–Organic Framework. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b04635
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