The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Fast Photoelectron Transfer in (Cring)–C3N4 Plane Heterostructural Nanosheets for Overall Water Splitting
Abstract
Direct and efficient photocatalytic water splitting is critical for sustainable conversion and storage of renewable solar energy. Here, we propose a conceptual design of two-dimensional C 3 N 4 -based in-plane heterostructure to achieve fast spatial transfer of photoexcited electrons for realizing highly efficient and spontaneous overall water splitting. This unique plane heterostructural carbon ring (C ring )–C 3 N 4 nanosheet can synchronously expedite electron–hole pair separation and promote photoelectron transport through the local in-plane π-conjugated electric field, synergistically elongating the photocarrier diffusion length and lifetime by 10 times relative to those achieved with pristine g-C 3 N 4 . As a result, the in-plane (C ring )–C 3 N 4 heterostructure could efficiently split pure water under light irradiation with prominent H 2 production rate up to 371 μmol g –1 h –1 and a notable quantum yield of 5% at 420 nm.
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Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Self-citationHydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Cited by
Cadmium sulfide-based nanomaterials for photocatalytic hydrogen production
Yuan, Y.-J., Chen, D., Yu, Z.-T., & Zou, Z.-G. (2018) · Journal of Materials Chemistry A · doi:10.1039/c8ta00671g · Cited by 523
2D Graphitic Carbon Nitride for Energy Conversion and Storage
Wang, Y., Liu, L., Ma, T., Zhang, Y., & Huang, H. (2021) · Advanced Functional Materials · doi:10.1002/adfm.202102540 · Cited by 448
Zhang, D., Guo, Y., & Zhao, Z. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2017.12.044 · Cited by 357
Xu, M., Lu, M., Qin, G., Wu, X., Yu, T., Zhang, L., Li, K., Cheng, X., & Lan, Y. (2022) · Angewandte Chemie International Edition · doi:10.1002/anie.202210700 · Cited by 319
Engineering β-ketoamine covalent organic frameworks for photocatalytic overall water splitting
Yang, Y., Chu, X., Zhang, H.-Y., Zhang, R., Liu, Y.-H., Zhang, F.-M., Lu, M., Yang, Z.-D., & Lan, Y.-Q. (2023) · Nature Communications · doi:10.1038/s41467-023-36338-x · Cited by 281
Metadata
- Authors
- Che, W., Cheng, W., Yao, T., Tang, F., Liu, W., Su, H., Huang, Y., Liu, Q., Liu, J., Hu, F., Pan, Z., Sun, Z., & Wei, S.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-02-21
- Volume
- 139
- Issue
- 8
- Pages
- 3021-3026
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2588349191
- Cited by
- 777
- References
- 3
- FWCI
- 23.20
- Type
- journal article
- Language
- en
- Open access
- closed
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- Che, W., Cheng, W., Yao, T., Tang, F., Liu, W., Su, H., Huang, Y., Liu, Q., Liu, J., Hu, F., Pan, Z., Sun, Z., & Wei, S. (2017). Fast Photoelectron Transfer in (Cring)–C3N4 Plane Heterostructural Nanosheets for Overall Water Splitting. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b11878
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