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RETRACTED: Metallic Conductivity in a Two-Dimensional Cobalt Dithiolene Metal–Organic Framework
Open accessAbstract
Two-dimensional (2D) metal-organic frameworks (MOFs) have received a great deal of attention due to their relatively high charge carrier mobility and low resistivity. Here we report on the temperature-dependent charge transport properties of a 2D cobalt 2,3,6,7,10,11-triphenylenehexathiolate framework. Variable temperature resistivity studies reveal a transition from a semiconducting to a metallic phase with decreasing temperature, which is unprecedented in MOFs. We find this transition to be highly dependent on the film thickness and the amount of solvent trapped in the pores, with density functional theory calculations of the electronic-structure supporting the complex metallic conductivity of the material. These results identify the first experimentally observed MOF that exhibits band-like metallic conductivity.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Earth-abundant catalysts for electrochemical and photoelectrochemical water splitting
Roger, I., Shipman, M. A., & Symes, M. D. (2017) · Nature Reviews Chemistry · doi:10.1038/s41570-016-0003 · Cited by 3,503
Cited by
Interface-Assisted Synthesis of 2D Materials: Trend and Challenges
Dong, R., Zhang, T., & Feng, X. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00056 · Cited by 710
Xu, G.-R., An, Z.-H., Xu, K., Liu, Q., Das, R., & Zhao, H.-L. (2021) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2020.213554 · Cited by 379
Metadata
- Authors
- Clough, A. J., Skelton, J. M., Downes, C. A., de la Rosa, A. A., Yoo, J. W., Walsh, A., Melot, B. C., & Marinescu, S. C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-13
- Volume
- 139
- Issue
- 31
- Pages
- 10863-10867
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2735584884
- Cited by
- 359
- References
- 2
- FWCI
- 15.22
- Type
- journal article
- Language
- en
- Status
- Retracted
- Open access
- green
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- Clough, A. J., Skelton, J. M., Downes, C. A., de la Rosa, A. A., Yoo, J. W., Walsh, A., Melot, B. C., & Marinescu, S. C. (2017). RETRACTED: Metallic Conductivity in a Two-Dimensional Cobalt Dithiolene Metal–Organic Framework. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.7b05742
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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