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Mesoporous Iron Sulfide for Highly Efficient Electrocatalytic Hydrogen Evolution
Open accessAbstract
We report a facile synthetic protocol to prepare mesoporous FeS 2 without the aid of hard template as an electrocatalyst for the hydrogen evolution reaction (HER). The mesoporous FeS 2 materials with high surface area were successfully prepared by a sol–gel method following a sulfurization treatment in an H 2 S atmosphere. A remarkable HER catalytic performance was achieved with a low overpotential of 96 mV at a current density of 10 mA·cm –2 and a Tafel slope of 78 mV per decade under alkaline conditions (pH 13). The theoretical calculations indicate that the excellent catalytic activity of mesoporous FeS 2 is attributed to the exposed (210) facets. The mesoporous FeS 2 material might be a promising alternative to the Pt-based electrocatalysts for water splitting.
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McCrory, C. C. L., Jung, S., Ferrer, I. M., Chatman, S. M., Peters, J. C., & Jaramillo, T. F. (2015) · Journal of the American Chemical Society · doi:10.1021/ja510442p · Cited by 4,145
Jin, H., Wang, J., Su, D., Wei, Z., Pang, Z., & Wang, Y. (2015) · Journal of the American Chemical Society · doi:10.1021/ja5127165 · Cited by 1,765
Gao, M.-R., Xu, Y.-F., Jiang, J., & Yu, S.-H. (2013) · Chemical Society Reviews · doi:10.1039/c2cs35310e · Cited by 1,610
Low Overpotential in Vacancy-Rich Ultrathin CoSe2 Nanosheets for Water Oxidation
Liu, Y., Cheng, H., Lyu, M., Fan, S., Liu, Q., Zhang, W., Zhi, Y., Wang, C., Xiao, C., Wei, S., et al. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5085157 · Cited by 1,094
First-row transition metal dichalcogenide catalysts for hydrogen evolution reaction
Kong, D., Cha, J. J., Wang, H., Lee, H. R., & Cui, Y. (2013) · Energy & Environmental Science · doi:10.1039/c3ee42413h · Cited by 1,031
Cited by
Nanoarchitectonics for Transition‐Metal‐Sulfide‐Based Electrocatalysts for Water Splitting
Guo, Y., Park, T., Yi, J. W., Henzie, J., Kim, J., Wang, Z., Jiang, B., Bando, Y., Sugahara, Y., Tang, J., et al. (2019) · Advanced Materials · doi:10.1002/adma.201807134 · Cited by 1,402
Recent progress in transition metal selenide electrocatalysts for water splitting
Xia, X., Wang, L., Sui, N., Colvin, V. L., & Yu, W. W. (2020) · Nanoscale · doi:10.1039/d0nr02939d · Cited by 336
Amorphous nanomaterials in electrocatalytic water splitting
Guo, C., Shi, Y., Lu, S., Yu, Y., & Zhang, B. (2021) · Chinese Journal of Catalysis · doi:10.1016/s1872-2067(20)63740-8 · Cited by 179
Li, Y., Tan, X., Tan, H., Ren, H., Chen, S., Yang, W., Smith, S. C., & Zhao, C. (2020) · Energy & Environmental Science · doi:10.1039/d0ee00666a · Cited by 133
Mohanty, B., Bhanja, P., & Jena, B. K. (2022) · Materials Today Energy · doi:10.1016/j.mtener.2021.100902 · Cited by 88
Metadata
- Authors
- Miao, R., Dutta, B., Sahoo, S., He, J., Zhong, W., Cetegen, S. A., Jiang, T., Alpay, S. P., & Suib, S. L.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-09-07
- Volume
- 139
- Issue
- 39
- Pages
- 13604-13607
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2753204810
- Cited by
- 344
- References
- 5
- FWCI
- 10.32
- Type
- journal article
- Language
- en
- Open access
- green
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- Miao, R., Dutta, B., Sahoo, S., He, J., Zhong, W., Cetegen, S. A., Jiang, T., Alpay, S. P., & Suib, S. L. (2017). Mesoporous Iron Sulfide for Highly Efficient Electrocatalytic Hydrogen Evolution. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.7b07044
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