The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Single-Atom Au/NiFe Layered Double Hydroxide Electrocatalyst: Probing the Origin of Activity for Oxygen Evolution Reaction
Abstract
Abstract A fundamental understanding of the origin of oxygen evolution reaction (OER) activity of transition-metal-based electrocatalysts, especially for single precious metal atoms supported on layered double hydroxides (LDHs), is highly required for the design of efficient electrocatalysts toward further energy conversion technologies. Here, we aim toward single-atom Au supported on NiFe LDH (sAu/NiFe LDH) to clarify the activity origin of LDHs system and a 6-fold OER activity enhancement by 0.4 wt % sAu decoration. Combining with theoretical calculations, the active behavior of NiFe LDH results from the in situ generated NiFe oxyhydroxide from LDH during the OER process. With the presence of sAu, sAu/NiFe LDH possesses an overpotential of 0.21 V in contrast to the calculated result (0.18 V). We ascribe the excellent OER activity of sAu/NiFe LDH to the charge redistribution of active Fe as well as its surrounding atoms causing by the neighboring sAu on NiFe oxyhydroxide stabilized by interfacial CO32– and H2O interfacing with LDH.
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Citations
Cites
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
Man, I. C., Su, H., Calle‐Vallejo, F., Hansen, H. A., Martínez, J. I., Inoglu, N. G., Kitchin, J., Jaramillo, T. F., Nørskov, J. K., & Rossmeisl, J. (2011) · ChemCatChem · doi:10.1002/cctc.201000397 · Cited by 4,769
Homogeneously dispersed multimetal oxygen-evolving catalysts
Zhang, B., Zheng, X., Voznyy, O., Comin, R., Bajdich, M., García-Melchor, M., Han, L., Xu, J., Liu, M., Zheng, L., et al. (2016) · Science · doi:10.1126/science.aaf1525 · Cited by 2,447
Self-citationJia, X., Zhao, Y., Chen, G., Shang, L., Shi, R., Kang, X., Waterhouse, G. I. N., Wu, L., Tung, C., & Zhang, T. (2016) · Advanced Energy Materials · doi:10.1002/aenm.201502585 · Cited by 773
Cited by
Li, P., Wang, M., Duan, X., Zheng, L., Cheng, X., Zhang, Y., Kuang, Y., Li, Y., Ma, Q., Feng, Z., et al. (2019) · Nature Communications · doi:10.1038/s41467-019-09666-0 · Cited by 717
Fe-Based Electrocatalysts for Oxygen Evolution Reaction: Progress and Perspectives
Feng, C., Faheem, M. B., Fu, J., Xiao, Y., Li, C., & Li, Y. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b05445 · Cited by 587
Single atom tungsten doped ultrathin α-Ni(OH)2 for enhanced electrocatalytic water oxidation
Yan, J., Kong, L., Ji, Y., White, J., Li, Y., Zhang, J., An, P., Liu, S., Lee, S.-T., & Ma, T. (2019) · Nature Communications · doi:10.1038/s41467-019-09845-z · Cited by 561
Self-citationDu, X., Huang, J., Zhang, J., Yan, Y., Wu, C., Hu, Y., Yan, C., Lei, T., Chen, W., Fan, C., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201810104 · Cited by 521
Self-citationHu, Y., Luo, G., Wang, L., Liu, X., Qu, Y., Zhou, Y., Zhou, F., Li, Z., Li, Y., Yao, T., et al. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202002816 · Cited by 423
Metadata
- Authors
- Zhang, J., Liu, J., Xi, L., Yu, Y., Chen, N., Sun, S., Wang, W., Lange, K. M., & Zhang, B.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-03-08
- Volume
- 140
- Issue
- 11
- Pages
- 3876-3879
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2792551382
- Cited by
- 1,034
- References
- 4
- FWCI
- 27.82
- Type
- journal article
- Language
- en
- Open access
- closed
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