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Space-Confined Strategy toward Large-Area Two-Dimensional Single Crystals of Molecular Materials
Abstract
Two-dimensional molecular crystals (2DMCs) are a promising candidate for flexible and large-area electronics. Their large-area production requires both low nuclei density and 2D crystal growth mode. As an emerging type of material, their large-area production remains a case-by-case practice. Here we present a general, efficient strategy for large-area 2DMCs. The method grows crystals on water surface to minimize the density of nuclei. By controlling the interfacial tension of the water/solution system with a phase transfer surfactant, the spreading area of the solvent increases tens of times, leading to the space-confined 2D growth of molecular crystals. As-grown sub-centimeter-sized 2DMCs floating on the water surface can be easily transferred to arbitrary substrates for device applications.
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Cites
Photonics and optoelectronics of 2D semiconductor transition metal dichalcogenides
Mak, K. F., & Shan, J. (2016) · Nature Photonics · doi:10.1038/nphoton.2015.282 · Cited by 3,819
Organic and Polymeric Semiconductors Enhanced by Noncovalent Conformational Locks
Huang, H., Yang, L., Facchetti, A., & Marks, T. J. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00084 · Cited by 804
Cited by
Organic crystalline materials in flexible electronics
Wang, Y., Sun, L., Wang, C., Yang, F., Ren, X., Zhang, X., Dong, H., & Hu, W. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00406d · Cited by 434
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Metadata
- Authors
- Wang, Q., Yang, F., Zhang, Y., Chen, M., Zhang, X., Lei, S., Li, R., & Hu, W.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-03-09
- Volume
- 140
- Issue
- 16
- Pages
- 5339-5342
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2790636744
- Cited by
- 176
- References
- 2
- FWCI
- 7.68
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, Q., Yang, F., Zhang, Y., Chen, M., Zhang, X., Lei, S., Li, R., & Hu, W. (2018). Space-Confined Strategy toward Large-Area Two-Dimensional Single Crystals of Molecular Materials. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.8b01997
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