The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Metal–Organic Framework Containing Planar Metal-Binding Sites: Efficiently and Cost-Effectively Enhancing the Kinetic Separation of C2H2/C2H4
Open accessAbstract
One of the emerging problems plaguing the chemical industry today is the efficient and cost-effective separation of C 2 hydrocarbons. In order to help address this problem, we report a new material, NbU-1, constructed by extremely cheap starting materials. The special structural characteristics of NbU-1 such as the planar, mixed-valence copper clusters and Lewis-basic adsorption channels enforce interactions with acetylene molecules that lead to the highest kinetic separation efficiency for C 2 H 2 /C 2 H 4 . Via DFT-D calculations, it is indicated that C 2 H 2 molecules are adsorbed onto the two adjacent Cu(I) centers, but not the usual single open metal sites of Cu centers. The reported results not only provide information for a deep investigation into the separation mechanism but also offer an alternative strategy for preparing cost-effective materials that can perform highly efficient separations of light hydrocarbons.
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Cites
Seven chemical separations to change the world
Sholl, D. S., & Lively, R. P. (2016) · Nature · doi:10.1038/532435a · Cited by 4,769
Control of zeolite framework flexibility and pore topology for separation of ethane and ethylene
Bereciartua, P. J., Cantín, Á., Corma, A., Jordá, J. L., Palomino, M., Rey, F., Valencia, S., Corcoran, E. W., Kortunov, P., Ravikovitch, P. I., et al. (2017) · Science · doi:10.1126/science.aao0092 · Cited by 460
Industrial Gas Handbook: Gas Separation and Purification
Kerry, F. G. (2007) · doi:10.1201/9781420008265 · Cited by 297
Cited by
Yang, L., Qian, S., Wang, X., Cui, X., Chen, B., & Xing, H. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00756c · Cited by 746
Optimizing Pore Space for Flexible-Robust Metal–Organic Framework to Boost Trace Acetylene Removal
Wang, J., Zhang, Y., Zhang, P., Hu, J., Lin, R.-B., Deng, Q., Zeng, Z., Xing, H., Deng, S., & Chen, B. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c02594 · Cited by 253
Metadata
- Authors
- Li, J., Jiang, L., Chen, S., Kirchon, A., Li, B., Li, Y., & Zhou, H.-C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-02-18
- Volume
- 141
- Issue
- 9
- Pages
- 3807-3811
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2911840138
- Cited by
- 206
- References
- 3
- FWCI
- 10.00
- Type
- journal article
- Language
- en
- Open access
- green
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- Li, J., Jiang, L., Chen, S., Kirchon, A., Li, B., Li, Y., & Zhou, H.-C. (2019). Metal–Organic Framework Containing Planar Metal-Binding Sites: Efficiently and Cost-Effectively Enhancing the Kinetic Separation of C2H2/C2H4. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.8b13463
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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