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A Photon Echo Peak Shift Study of Liquid Water
Abstract
The first photon echo peak shift study of liquid water is presented. Spectral diffusion within the OH stretching absorption band of HDO in D 2 O takes place on many time scales with a slow component on the order of 5−15 ps. This indicates that fluctuations of local structure of the hydrogen bond network in liquid water are relatively long-lived. Vibrational relaxation of the excited state populates a state which is spectroscopically different from the initial ground state. This leads to an strong enhancement of the peak shift and allows spectral diffusion to be measured for delay times beyond the limit determined by the population relaxation time T 1 . The observed signals are discussed with the help of model calculations.
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Cites
Ultrafast Energy Transfer in LHC-II Revealed by Three-Pulse Photon Echo Peak Shift Measurements
Agarwal, R., Krueger, B. P., Scholes, G. D., Yang, M., Yom, J., Mets, L., & Fleming, G. R. (2000) · The Journal of Physical Chemistry B · doi:10.1021/jp9915578 · Cited by 114
Cited by
Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Vibrational Spectroscopic Map, Vibrational Spectroscopy, and Intermolecular Interaction
Baiz, C. R., Błasiak, B., Bredenbeck, J., Cho, M., Choi, J.-H., Corcelli, S. A., Dijkstra, A. G., Feng, C.-J., Garrett-Roe, S., Ge, N.-H., et al. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00813 · Cited by 412
Structure, Dynamics, and Spectral Diffusion of Water from First-Principles Molecular Dynamics
Bankura, A., Karmakar, A., Carnevale, V., Chandra, A., & Klein, M. L. (2014) · The Journal of Physical Chemistry C · doi:10.1021/jp506120t · Cited by 166
Metadata
- Authors
- Stenger, J., Madsen, D., Hamm, P., Nibbering, E. T. J., & Elsaesser, T.
- Venue
- The Journal of Physical Chemistry A
- Publisher
- American Chemical Society (ACS)
- Published
- 2002-01-29
- Volume
- 106
- Issue
- 10
- Pages
- 2341-2350
- ISSN
- 1089-5639 (ISSN-L)
- 1520-5215
- OpenAlex
- W2072225167
- Cited by
- 208
- References
- 1
- FWCI
- 15.67
- Type
- journal article
- Language
- en
- Open access
- closed
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- Stenger, J., Madsen, D., Hamm, P., Nibbering, E. T. J., & Elsaesser, T. (2002). A Photon Echo Peak Shift Study of Liquid Water. The Journal of Physical Chemistry A. https://doi.org/10.1021/jp013104k
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