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Hydrogen Bond Dynamics in Water and Ultrafast Infrared Spectroscopy
Abstract
Molecular dynamics simulations are used to examine two key aspects of recent ultrafast infrared experiments on liquid water dynamics. It is found that the relation between the OH stretch frequency and the length of the hydrogen bond in which the OH is involved, currently assumed to be one-to-one, is instead characterized by considerable dispersion and that the time scale currently interpreted in terms of a stochastic modulation by the surrounding solvent of a highly frictionally damped hydrogen bond system is shown to be governed by hydrogen bond-breaking and -making dynamics, whereas the motion of an intact hydrogen-bonded complex is underdamped in character.
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Cited by
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Jonas, D. M. (2003) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.54.011002.103907 · Cited by 1,198
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Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Hydrogen bonding at the water surface revealed by isotopic dilution spectroscopy
Stiopkin, I. V., Weeraman, C., Pieniazek, P. A., Shalhout, F. Y., Skinner, J. L., & Benderskii, A. V. (2011) · Nature · doi:10.1038/nature10173 · Cited by 462
On the Molecular Mechanism of Water Reorientation
Laage, D., & Hynes, J. T. (2008) · The Journal of Physical Chemistry B · doi:10.1021/jp805217u · Cited by 438
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Metadata
- Authors
- Rey, R., Møller, K. B., & Hynes, J. T.
- Venue
- The Journal of Physical Chemistry A
- Publisher
- American Chemical Society (ACS)
- Published
- 2002-11-22
- Volume
- 106
- Issue
- 50
- Pages
- 11993-11996
- ISSN
- 1089-5639 (ISSN-L)
- 1520-5215
- OpenAlex
- W2005309347
- Cited by
- 344
- References
- 0
- FWCI
- 12.09
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rey, R., Møller, K. B., & Hynes, J. T. (2002). Hydrogen Bond Dynamics in Water and Ultrafast Infrared Spectroscopy. The Journal of Physical Chemistry A. https://doi.org/10.1021/jp026419o
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