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Optical Properties of Metal Nanoshells
Abstract
We present a combination of theory and experiment designed to elucidate the properties of gold nanoshells. Wet chemistry methods are used to prepare the nanoshells, and transmission electron microscopy (TEM) analysis is used to characterize the shell structure, demonstrating the presence of pinholes in the shells. Both Mie theory and the discrete dipole approximation (a numerical method) are used to characterize the electrodynamics of the shell structures, including both perfect and pinhole defected shells. The calculations show that 2−5 nm pinholes have only a small effect on the extinction spectra; however, they lead to local electric fields that are enhanced by a factor of 3−4 close to the plasmon maximum. This makes metal nanoshells (with holes) attractive materials for surface enhanced Raman spectroscopy applications.
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Cites
Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen
Mie, G. (1908) · Annalen der Physik · doi:10.1002/andp.19083300302 · Cited by 11,537
Cited by
Exploitation of Localized Surface Plasmon Resonance
Hutter, E., & Fendler, J. H. (2004) · Advanced Materials · doi:10.1002/adma.200400271 · Cited by 2,726
Shape‐Controlled Synthesis of Metal Nanostructures: The Case of Silver
Wiley, B., Sun, Y., Mayers, B., & Xia, Y. (2005) · Chemistry – A European Journal · doi:10.1002/chem.200400927 · Cited by 1,643
Templated Techniques for the Synthesis and Assembly of Plasmonic Nanostructures
Jones, M. R., Osberg, K. D., Macfarlane, R. J., Langille, M. R., & Mirkin, C. A. (2011) · Chemical Reviews · doi:10.1021/cr1004452 · Cited by 1,159
Nanoparticle colloidal stability in cell culture media and impact on cellular interactions
Moore, T. L., Rodriguez-Lorenzo, L., Hirsch, V., Balog, S., Urban, D., Jud, C., Rothen-Rutishauser, B., Lattuada, M., & Petri-Fink, A. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00487f · Cited by 1,082
Synthesis and Optical Properties of Anisotropic Metal Nanoparticles
Hao, E., Schatz, G. C., & Hupp, J. T. (2004) · Journal of Fluorescence · doi:10.1023/b:jofl.0000031815.71450.74 · Cited by 312
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Metadata
- Authors
- Hao, E., Li, S., Bailey, R. C., Zou, S., Schatz, G. C., & Hupp, J. T.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-01-01
- Volume
- 108
- Issue
- 4
- Pages
- 1224-1229
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W2085866590
- Cited by
- 288
- References
- 1
- FWCI
- 11.09
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hao, E., Li, S., Bailey, R. C., Zou, S., Schatz, G. C., & Hupp, J. T. (2004). Optical Properties of Metal Nanoshells. The Journal of Physical Chemistry B. https://doi.org/10.1021/jp036301n
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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