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Effect of Chemical Treatment on Electrical Conductivity, Infrared Absorption, and Raman Spectra of Single-Walled Carbon Nanotubes
Abstract
We investigate the magnitude and temperature dependence of electrical conductivity, the optical and infrared absorption, and the Raman spectra of single-walled carbon nanotube (SWNT) bucky-paper after chemical treatment and determine the correlations between the changes in these properties. Ionic-acceptor doping of the SWNT bucky-paper (with SOCl(2), iodine, H(2)SO(3), etc.) causes an increase of electrical conductivity that correlates with an increase of the absorbance in the far-IR region and an increase in the frequency of Raman spectral lines. Conversely, treatment with other molecules (e.g., aniline, PyPhF(5), PhCH(2)Br, etc.) leads to a decrease in both conductivity and far-IR absorption. The temperature dependence of the conductivity gives a good indication of the presence of metallic charge carriers and is in agreement with the model of interrupted metallic conduction.
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Cited by
Aqueous Suspension and Characterization of Chemically Modified Graphene Sheets
Park, S., An, J., Piner, R. D., Jung, I., Yang, D., Velamakanni, A., Nguyen, S. T., & Ruoff, R. S. (2008) · Chemistry of Materials · doi:10.1021/cm801932u · Cited by 965
Xue, X., Wang, L.-R., Sato, Y., Jiang, Y., Berg, M., Yang, D.-S., Nixon, R. A., & Liang, X.-J. (2014) · Nano Letters · doi:10.1021/nl501839q · Cited by 125
Metadata
- Authors
- Skákalová, V., Kaiser, A. B., Dettlaff-Weglikowska, U., Hrnčariková, K., & Roth, S.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-03-19
- Volume
- 109
- Issue
- 15
- Pages
- 7174-7181
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W2048120351
- Cited by
- 219
- References
- 0
- FWCI
- 9.07
- Type
- journal article
- Language
- en
- Open access
- closed
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- Skákalová, V., Kaiser, A. B., Dettlaff-Weglikowska, U., Hrnčariková, K., & Roth, S. (2005). Effect of Chemical Treatment on Electrical Conductivity, Infrared Absorption, and Raman Spectra of Single-Walled Carbon Nanotubes. The Journal of Physical Chemistry B. https://doi.org/10.1021/jp044741o
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