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Cited by 205

The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.

Heterogeneous Surface Crystallization Observed in Undercooled Water

Shaw, Raymond A., Durant, Adam J., Mi, Youshi·2005·The Journal of Physical Chemistry B

Abstract

We report laboratory observations of higher freezing temperatures when an ice-forming nucleus is near the surface of an undercooled water drop than when the nucleus is immersed in the drop. The nucleation rate at the water surface is a factor of 10(10) greater than in bulk water, thereby complementing and providing evidence for homogeneous surface crystallization, which has been hypothesized recently. Interpretation of the data via classical nucleation theory shows that the free energy of formation of a critical ice germ is decreased by a factor of approximately 2 when the substrate is near the air-water interface. Furthermore, the analysis suggests that the jump frequency of molecules from the liquid to the solid may be greatly enhanced at the interface.

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Crossref · 10.1021/jp0506336

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Metadata

Authors
Shaw, R. A., Durant, A. J., & Mi, Y.
Venue
The Journal of Physical Chemistry B
Published
2005-05-01
Volume
109
Issue
20
Pages
9865-9868
ISSN
  • 1520-5207 (ISSN-L)
  • 1520-6106
OpenAlex
W2037307077
Cited by
205
References
1
FWCI
4.69
Type
journal article
Language
en
Open access
closed

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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