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Overall Water Splitting on (Ga1-xZnx)(N1-xOx) Solid Solution Photocatalyst: Relationship between Physical Properties and Photocatalytic Activity
Abstract
The physical and photocatalytic properties of a novel solid solution between GaN and ZnO, (Ga(1-x)Zn(x))(N(1-x)O(x)), are investigated. Nitridation of a mixture of Ga(2)O(3) and ZnO at 1123 K for 5-30 h under NH(3) flow results in the formation of a (Ga(1-x)Zn(x))(N(1-x)O(x)) solid solution with x = 0.05-0.22. With increasing nitridation time, the zinc and oxygen concentrations decrease due to reduction of ZnO and volatilization of zinc, and the crystallinity and band gap energy of the product increase. The highest activity for overall water splitting is obtained for (Ga(1-x)Zn(x))(N(1-x)O(x)) with x = 0.12 after nitridation for 15 h. The crystallinity of the catalyst is also found to increase with increasing the ratio of ZnO to Ga(2)O(3) in the starting material, resulting in an increase in activity.
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Shannon, R. D. (1976) · Acta Crystallographica Section A · doi:10.1107/s0567739476001551 · Cited by 66,145
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Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
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Kubacka, A., Fernández-García, M., & Colón, G. (2012) · Chemical Reviews · doi:10.1021/cr100454n · Cited by 2,373
Abe, R. (2010) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2011.02.003 · Cited by 1,223
Maeda, K., Teramura, K., Lu, D., Saito, N., Inoue, Y., & Domen, K. (2006) · Angewandte Chemie International Edition · doi:10.1002/anie.200602473 · Cited by 641
Self-citationChen, G., Li, D., Li, F., Fan, Y., Zhao, H., Luo, Y., Yu, R., & Meng, Q. (2012) · Applied Catalysis A: General · doi:10.1016/j.apcata.2012.07.033 · Cited by 154
Metadata
- Authors
- Maeda, K., Teramura, K., Takata, T., Hara, M., Saito, N., Toda, K., Inoue, Y., Kobayashi, H., & Domen, K.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-10-01
- Volume
- 109
- Issue
- 43
- Pages
- 20504-20510
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W2052774499
- Cited by
- 389
- References
- 1
- FWCI
- 11.21
- Type
- journal article
- Language
- en
- Open access
- closed
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