The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Imaging Water Dissociation on TiO2(110): Evidence for Inequivalent Geminate OH Groups
Abstract
Identical regions of partially reduced TiO2(110) surfaces with bridge-bonded oxygen vacancy (BBO(V)) concentrations of approximately 10% ML (1 ML = 5.2 x 10(14) cm(-2)) were imaged using scanning tunneling microscopy (STM) before and after dosing H2O at ambient temperature (approximately 300 K). Atomically resolved images confirm that H2O adsorbs dissociatively on the BBO(V) sites, producing two hydroxyl species, one positioned at BBO(V) and denoted OH(V) and the other, denoted OH(B), formed by protonation at either of the two nearest-neighbor bridge-bonded oxygen atoms. Hydrogen hopping along the [001] direction is observed at ambient temperature, with a strong preference for OH(B) (approximately 10x) hydrogen motion. This powerful imbalance demonstrates the inequality of OH(V) and OH(B) and suggests differences in their charge and/or binding configuration.
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Cites
The surface science of titanium dioxide
Diebold, U. (2003) · Surface Science Reports · doi:10.1016/s0167-5729(02)00100-0 · Cited by 7,944
All-boron aromatic clusters as potential new inorganic ligands and building blocks in chemistry
Alexandrova, A. N., Boldyrev, A. I., Zhai, H.-J., & Wang, L.-S. (2006) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2006.03.032 · Cited by 712
Cited by
TiO2 photocatalysis and related surface phenomena
FUJISHIMA, A., ZHANG, X., & TRYK, D. (2008) · Surface Science Reports · doi:10.1016/j.surfrep.2008.10.001 · Cited by 6,737
Fundamentals of TiO2 Photocatalysis: Concepts, Mechanisms, and Challenges
Guo, Q., Zhou, C., Ma, Z., & Yang, X. (2019) · Advanced Materials · doi:10.1002/adma.201901997 · Cited by 1,909
In situ x-ray photoelectron spectroscopy studies of water on metals and oxides at ambient conditions
Yamamoto, S., Bluhm, H., Andersson, K., Ketteler, G., Ogasawara, H., Salmeron, M., & Nilsson, A. (2008) · Journal of Physics: Condensed Matter · doi:10.1088/0953-8984/20/18/184025 · Cited by 314
Thermally-driven processes on rutile TiO2(110)-(1×1): A direct view at the atomic scale
Dohnálek, Z., Lyubinetsky, I., & Rousseau, R. (2010) · Progress in Surface Science · doi:10.1016/j.progsurf.2010.03.001 · Cited by 310
Self-citationDistribution of Ti3+ Surface Sites in Reduced TiO2
Deskins, N. A., Rousseau, R., & Dupuis, M. (2011) · The Journal of Physical Chemistry C · doi:10.1021/jp2001139 · Cited by 267
Metadata
- Authors
- Zhang, Z., Bondarchuk, O., Kay, B. D., White, J. M., & Dohnálek, Z.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-10-04
- Volume
- 110
- Issue
- 43
- Pages
- 21840-21845
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W1979778096
- Cited by
- 229
- References
- 2
- FWCI
- 12.53
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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