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The Nature of Water Nucleation Sites on TiO2(110) Surfaces Revealed by Ambient Pressure X-ray Photoelectron Spectroscopy
Open accessAbstract
X-ray photoelectron spectroscopy at ambient conditions of pressure (up to 1.5 Torr) and temperature (265 K < T < 800 K) was used to study the adsorption of water on rutile TiO 2 (110) under conditions of thermodynamic equilibrium. It was found that OH groups in bridging positions, normally present in small amounts due to residual O-vacancies, act as nucleation sites for subsequent water adsorption. The adsorption enthalpy of water binding to these sites is ∼70 kJ/mol, much stronger than that in the bulk liquid (45 kJ/mol). A model is proposed that relates the structure of the oxide surface to its hydrophilic character.
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Citations
Cites
Electrochemical Photolysis of Water at a Semiconductor Electrode
FUJISHIMA, A., & HONDA, K. (1972) · Nature · doi:10.1038/238037a0 · Cited by 34,169
The surface science of titanium dioxide
Diebold, U. (2003) · Surface Science Reports · doi:10.1016/s0167-5729(02)00100-0 · Cited by 7,944
Cited by
Water-Mediated Promotion of Dye Sensitization of TiO2 under Visible Light
Pan, L., Zou, J.-J., Zhang, X., & Wang, L. (2011) · Journal of the American Chemical Society · doi:10.1021/ja2035927 · Cited by 258
Direction-specific van der Waals attraction between rutile TiO 2 nanocrystals
Zhang, X., He, Y., Sushko, M. L., Liu, J., Luo, L., De Yoreo, J. J., Mao, S. X., Wang, C., & Rosso, K. M. (2017) · Science · doi:10.1126/science.aah6902 · Cited by 122
Metadata
- Authors
- Ketteler, G., Yamamoto, S., Bluhm, H., Andersson, K., Starr, D. E., Ogletree, D. F., Ogasawara, H., Nilsson, A., & Salmeron, M.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-05-17
- Volume
- 111
- Issue
- 23
- Pages
- 8278-8282
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2009701080
- Cited by
- 419
- References
- 2
- FWCI
- 7.98
- Type
- journal article
- Language
- en
- Open access
- green
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- Ketteler, G., Yamamoto, S., Bluhm, H., Andersson, K., Starr, D. E., Ogletree, D. F., Ogasawara, H., Nilsson, A., & Salmeron, M. (2007). The Nature of Water Nucleation Sites on TiO2(110) Surfaces Revealed by Ambient Pressure X-ray Photoelectron Spectroscopy. The Journal of Physical Chemistry C. https://doi.org/10.1021/jp068606i
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