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Surface Enhanced Raman Scattering Enhancement Factors: A Comprehensive Study
Abstract
This paper presents an in-depth study of Surface Enhanced Raman Scattering (SERS) enhancement factors (EFs) and cross-sections, including several issues often overlooked. In particular, various possible rigorous definitions of the SERS EFs are introduced and discussed in the context of SERS applications, such as analytical chemistry and single molecule SERS. These definitions highlight the importance of a careful characterization of the non-SERS cross-sections of the probes under consideration. This aspect is illustrated by experimental results for the non-SERS cross-sections of representative SERS probes along with average SERS EFs for the same probes. In addition, the accurate experimental determination of single molecule enhancement factors is tackled with two recently developed techniques, namely: bi-analyte SERS (BiASERS) and temperature-dependent SERS vibrational pumping. We demonstrate that SERS EFs as low as 10 7, as opposed to the figure of 10 14 often claimed in the literature, are sufficient for the observation of single molecule SERS signals, with maximum single molecule EFs typically on the order of ∼10 10 .
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Cites
Raman spectra of pyridine adsorbed at a silver electrode
Fleischmann, M., Hendra, P. J., & McQuillan, A. J. (1974) · Chemical Physics Letters · doi:10.1016/0009-2614(74)85388-1 · Cited by 7,172
Surface raman spectroelectrochemistry
Jeanmaire, D. L., & Van Duyne, R. P. (1977) · Journal of Electroanalytical Chemistry and Interfacial Electrochemistry · doi:10.1016/s0022-0728(77)80224-6 · Cited by 4,738
Cited by
Gold Nanorods: From Synthesis and Properties to Biological and Biomedical Applications
Huang, X., Neretina, S., & El‐Sayed, M. A. (2009) · Advanced Materials · doi:10.1002/adma.200802789 · Cited by 1,921
Localized surface plasmon resonance: Nanostructures, bioassays and biosensing—A review
Petryayeva, E., & Krull, U. J. (2011) · Analytica Chimica Acta · doi:10.1016/j.aca.2011.08.020 · Cited by 1,379
Fan, M., Andrade, G. F. S., & Brolo, A. G. (2020) · Analytica Chimica Acta · doi:10.1016/j.aca.2019.11.049 · Cited by 533
Single molecule analysis by surfaced-enhanced Raman scattering
Pieczonka, N. P. W., & Aroca, R. F. (2008) · Chemical Society Reviews · doi:10.1039/b709739p · Cited by 451
Guerrini, L., & Graham, D. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35118h · Cited by 441
Metadata
- Authors
- Le Ru, E. C., Blackie, E., Meyer, M., & Etchegoin, P. G.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-08-23
- Volume
- 111
- Issue
- 37
- Pages
- 13794-13803
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2092049851
- Cited by
- 2,853
- References
- 2
- FWCI
- 28.94
- Type
- journal article
- Language
- en
- Open access
- closed
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