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Comparison of the Oxygen Reduction Reaction between NaOH and KOH Solutions on a Pt Electrode: The Electrolyte-Dependent Effect
Open accessAbstract
The oxygen reduction reaction (ORR) on a polycrystalline Pt surface was studied using cyclic voltammetry techniques, and the influence of reaction media on the ORR is examined by comparing the ORR in NaOH and KOH solutions with concentration ranging from 0.5 to 14 M at 298 K. The results show that, in NaOH and KOH solutions, the ORR, a quasi-reversible diffusion-controlled reaction, is largely dependent on the electrolyte conditions, and KOH solutions are superior to NaOH solutions for the ORR process in both thermodynamic and kinetic consideration. As the alkaline concentration increases, the ORR performance frustrates, and the protonation of superoxide is suppressed; thus, the ORR shifts from a 2e reduction pathway to a 1e reduction pathway in both solutions.
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Cites
Oxygen Reduction on Carbon-Supported Pt−Ni and Pt−Co Alloy Catalysts
Paulus, U. A., Wokaun, A., Scherer, G. G., Schmidt, T. J., Stamenkovic, V., Radmilovic, V., Markovic, N. M., & Ross, P. N. (2002) · The Journal of Physical Chemistry B · doi:10.1021/jp013442l · Cited by 954
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Mukerjee, S., Srinivasan, S., Soriaga, M. P., & McBreen, J. (1995) · The Journal of Physical Chemistry · doi:10.1021/j100013a032 · Cited by 439
Importance of Interatomic Spacing in Catalytic Reduction of Oxygen in Phosphoric Acid
Jalan, V., & Taylor, E. J. (1983) · Journal of The Electrochemical Society · doi:10.1149/1.2119574 · Cited by 363
In Situ X‐Ray Absorption Studies of a Pt‐Ru Electrocatalyst
McBreen, J., & Mukerjee, S. (1995) · Journal of The Electrochemical Society · doi:10.1149/1.2049993 · Cited by 242
Activation Energies for Oxygen Reduction on Platinum Alloys: Theory and Experiment
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Pan, J., Xu, Y. Y., Yang, H., Dong, Z., Liu, H., & Xia, B. Y. (2018) · Advanced Science · doi:10.1002/advs.201700691 · Cited by 848
Developments in electrode materials and electrolytes for aluminium–air batteries
Egan, D. R., Ponce de León, C., Wood, R. J. K., Jones, R. L., Stokes, K. R., & Walsh, F. C. (2013) · Journal of Power Sources · doi:10.1016/j.jpowsour.2013.01.141 · Cited by 465
Zhu, H., Zhang, S., Huang, Y.-X., Wu, L., & Sun, S. (2013) · Nano Letters · doi:10.1021/nl401325u · Cited by 462
Lin, Z., Waller, G. H., Liu, Y., Liu, M., & Wong, C.-P. (2013) · Nano Energy · doi:10.1016/j.nanoen.2012.09.002 · Cited by 395
Ribeiro, E. L., Davis, E. M., Mokhtarnejad, M., Hu, S., Mukherjee, D., & Khomami, B. (2021) · Catalysis Science & Technology · doi:10.1039/d0cy02099k · Cited by 34
Metadata
- Authors
- Jin, W., Du, H., Zheng, S., Xu, H., & Zhang, Y.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-04-22
- Volume
- 114
- Issue
- 19
- Pages
- 6542-6548
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W1984950720
- Cited by
- 184
- References
- 6
- FWCI
- 4.00
- Type
- journal article
- Language
- en
- Open access
- green
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