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Visible Light Photocatalysis of BiOI and Its Photocatalytic Activity Enhancement by in Situ Ionic Liquid Modification
Abstract
In this study, we investigate the photocatalysis mechanism of BiOI in detail and therefore demonstrate that the photocatalytic activity of BiOI could be enhanced greatly by in situ modification of an ionic liquid [Bmim]I (1-buty-3-methylimidazolium iodide). The ionic liquid modified BiOI (IL-BiOI) was prepared by reacting bismuth nitrate with [Bmim]I in water at 70 °C, where the ionic liquid could act as both iodine source and surface modified agent. On degradation of methyl orange (MO) under visible light irradiation (λ > 420 nm), IL-BiOI photocatalyst exhibited superior photocatalytic activity to the unmodified counterpart synthesized in the absence of [Bmim]I. The effects of ionic liquid modification on the photocatalytic activity enhancement were systematically investigated. We found that IL modification could trap the photoexcited electron at conduction band of BiOI to inhibit the recombination of photoinduced electron–hole pairs and thus enhance its photocatalytic activity on the degradation of organic pollutants.
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Buxton, G. V., Greenstock, C. L., Helman, W. P., & Ross, A. B. (1988) · Journal of Physical and Chemical Reference Data · doi:10.1063/1.555805 · Cited by 12,332
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Engineering BiOX (X = Cl, Br, I) nanostructures for highly efficient photocatalytic applications
Cheng, H., Huang, B., & Dai, Y. (2014) · Nanoscale · doi:10.1039/c3nr05529a · Cited by 1,119
Sharma, K., Dutta, V., Sharma, S., Raizada, P., Hosseini-Bandegharaei, A., Thakur, P., & Singh, P. (2019) · Journal of Industrial and Engineering Chemistry · doi:10.1016/j.jiec.2019.06.022 · Cited by 391
Facile in situ synthesis of a Bi/BiOCl nanocomposite with high photocatalytic activity
Weng, S., Chen, B., Xie, L., Zheng, Z., & Liu, P. (2013) · Journal of Materials Chemistry A · doi:10.1039/c2ta01004f · Cited by 358
Chang, C., Zhu, L., Wang, S., Chu, X., & Yue, L. (2014) · ACS Applied Materials & Interfaces · doi:10.1021/am5002597 · Cited by 326
Metadata
- Authors
- Wang, Y., Deng, K., & Zhang, L.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-07-06
- Volume
- 115
- Issue
- 29
- Pages
- 14300-14308
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2320675731
- Cited by
- 292
- References
- 1
- FWCI
- 10.25
- Type
- journal article
- Language
- en
- Open access
- closed
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