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Electrochemical Activity of Black Phosphorus as an Anode Material for Lithium-Ion Batteries
Abstract
Black phosphorus (black P), which is a promising candidate as an anode material for lithium-ion batteries, was synthesized by a high-pressure and high-temperature (HPHT) method from white and red phosphorus. The study revealed the electrochemical activity of pure black P under different pressures and temperatures systematically. The sample shows higher crystallinity and purity by the HPHT method. Lithium-ion batteries containing black phosphorus as anode materials exhibited a high specific capacity and excellent cycling performance. Black phosphorus obtained from white phosphorus exhibited the highest first discharge and charge capacities of 2505 and 1354 mAh·g –1 at 4 GPa and 400 °C and that obtained from red phosphorus exhibited the highest first discharge and charge capacities of 2649 and 1425 mAh·g –1 at 4.5 GPa and 800 °C. Black P was characterized by X-ray diffraction, Raman microscopy, scanning electron microscopy, and high-resolution transmission electron microscopy.
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Citations
Cited by
An Amorphous Red Phosphorus/Carbon Composite as a Promising Anode Material for Sodium Ion Batteries
Kim, Y., Park, Y., Choi, A., Choi, N., Kim, J., Lee, J., Ryu, J. H., Oh, S. M., & Lee, K. T. (2013) · Advanced Materials · doi:10.1002/adma.201204877 · Cited by 854
Li, W., Yang, Y., Zhang, G., & Zhang, Y.-W. (2015) · Nano Letters · doi:10.1021/nl504336h · Cited by 773
Zhang, X., Xie, H., Liu, Z., Tan, C., Luo, Z., Li, H., Lin, J., Sun, L., Chen, W., Xu, Z., et al. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201409400 · Cited by 710
Self-citationNegative electrodes for Na-ion batteries
Dahbi, M., Yabuuchi, N., Kubota, K., Tokiwa, K., & Komaba, S. (2014) · Physical Chemistry Chemical Physics · doi:10.1039/c4cp00826j · Cited by 623
Applications of Phosphorene and Black Phosphorus in Energy Conversion and Storage Devices
Pang, J., Bachmatiuk, A., Yin, Y., Trzebicka, B., Zhao, L., Fu, L., Mendes, R. G., Gemming, T., Liu, Z., & Rummeli, M. H. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702093 · Cited by 518
Metadata
- Authors
- Sun, L.-Q., Li, M.-J., Sun, K., Yu, S.-H., Wang, R.-S., & Xie, H.-M.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-07-03
- Volume
- 116
- Issue
- 28
- Pages
- 14772-14779
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2044975616
- Cited by
- 293
- References
- 0
- FWCI
- 9.56
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sun, L.-Q., Li, M.-J., Sun, K., Yu, S.-H., Wang, R.-S., & Xie, H.-M. (2012). Electrochemical Activity of Black Phosphorus as an Anode Material for Lithium-Ion Batteries. The Journal of Physical Chemistry C. https://doi.org/10.1021/jp302265n
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