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Electrochemical Synthesis of Very Stable Photoluminescent Copper Clusters
Abstract
Small fluorescent atomic copper clusters, stabilized by tetrabutylammonium nitrate, have been synthesized by a simple electrochemical technique. These small clusters (Cu N, N < ≈14) show photoluminescence in the visible range with unusual high quantum yields (13%) and were characterized by UV−vis and fluorescence spectroscopies, LDI-TOF (laser desorption/ionization time-of-flight) mass spectroscopy, XPS (X-ray photoelectron spectroscopy), and TEM/HRTEM (high-resolution/transmission electron microscopy). Cu clusters are very stable and can be dispersed in both apolar and polar solvents, which makes them useful as very small building blocks, bringing new possibilities to construct novel nano/microstructures, with potential applications in fields such as biosensors, biomedicine, etc.
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Cites
Identification of Active Gold Nanoclusters on Iron Oxide Supports for CO Oxidation
Herzing, A. A., Kiely, C. J., Carley, A. F., Landon, P., & Hutchings, G. J. (2008) · Science · doi:10.1126/science.1159639 · Cited by 1,530
Cited by
Sub-nanometre sized metal clusters: from synthetic challenges to the unique property discoveries
Lu, Y., & Chen, W. (2012) · Chemical Society Reviews · doi:10.1039/c2cs15325d · Cited by 1,152
New trends in tailoring active sites in zeolite-based catalysts
Shamzhy, M., Opanasenko, M., Concepción, P., & Martínez, A. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00887f · Cited by 508
Wei, W., Lu, Y., Chen, W., & Chen, S. (2011) · Journal of the American Chemical Society · doi:10.1021/ja109303z · Cited by 481
Jia, X., Yang, X., Li, J., Li, D., & Wang, E. (2014) · Chem. Commun. · doi:10.1039/c3cc47771a · Cited by 332
Atomically precise copper nanoclusters and their applications
Liu, X., & Astruc, D. (2018) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2018.01.001 · Cited by 322
Metadata
- Authors
- Vilar-Vidal, N., Blanco, M. C., López-Quintela, M. A., Rivas, J., & Serra, C.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-07-26
- Volume
- 114
- Issue
- 38
- Pages
- 15924-15930
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2040933290
- Cited by
- 217
- References
- 1
- FWCI
- 4.79
- Type
- journal article
- Language
- en
- Open access
- closed
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- Vilar-Vidal, N., Blanco, M. C., López-Quintela, M. A., Rivas, J., & Serra, C. (2010). Electrochemical Synthesis of Very Stable Photoluminescent Copper Clusters. The Journal of Physical Chemistry C. https://doi.org/10.1021/jp911380s
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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