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Supercooled Liquids and Glasses
Abstract
Selected aspects of recent progress in the study of supercooled liquids and glasses are presented in this review. As an introduction for nonspecialists, several basic features of the dynamics and thermodynamics of supercooled liquids and glasses are described. Among these are nonexponential relaxation functions, non-Arrhenius temperature dependences, and the Kauzmann temperature. Various theoretical models which attempt to explain these basic features are presented next. These models are conveniently categorized according to the temperature regimes deemed important by their authors. The major portion of this review is given to a summary of current experimental and computational research. The utility of mode coupling theory is addressed. Evidence is discussed for new relaxation mechanisms and new time and length scales in supercooled liquids. Relaxations in the glassy state and significance of the “boson peak” are also addressed.
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Cites
Thermal Conductivity and Specific Heat of Noncrystalline Solids
Zeller, R. C., & Pohl, R. O. (1971) · Physical Review B · doi:10.1103/physrevb.4.2029 · Cited by 1,954
Cited by
Characteristics and Significance of the Amorphous State in Pharmaceutical Systems
Hancock, B. C., & Zografi, G. (1997) · Journal of Pharmaceutical Sciences · doi:10.1021/js9601896 · Cited by 1,922
Atomic-level structure and structure–property relationship in metallic glasses
Cheng, Y. Q., & Ma, E. (2011) · Progress in Materials Science · doi:10.1016/j.pmatsci.2010.12.002 · Cited by 1,771
Denissen, W., Rivero, G., Nicolaÿ, R., Leibler, L., Winne, J. M., & Du Prez, F. E. (2015) · Advanced Functional Materials · doi:10.1002/adfm.201404553 · Cited by 1,121
Structural heterogeneities and mechanical behavior of amorphous alloys
Qiao, J. C., Wang, Q., Pelletier, J. M., Kato, H., Casalini, R., Crespo, D., Pineda, E., Yao, Y., & Yang, Y. (2019) · Progress in Materials Science · doi:10.1016/j.pmatsci.2019.04.005 · Cited by 659
Laughlin, R. B., Pines, D., Schmalian, J., Stojković, B. P., & Wolynes, P. (2000) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.97.1.32 · Cited by 391
Metadata
- Authors
- Ediger, M. D., Angell, C. A., & Nagel, S. R.
- Venue
- The Journal of Physical Chemistry
- Publisher
- American Chemical Society (ACS)
- Published
- 1996-01-01
- Volume
- 100
- Issue
- 31
- Pages
- 13200-13212
- ISSN
- 0022-3654 (ISSN-L)
- 1541-5740
- OpenAlex
- W2158036413
- Cited by
- 2,220
- References
- 1
- FWCI
- 61.82
- Type
- journal article
- Language
- en
- Open access
- closed
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