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Interparticle Electron Transfer in Metal/Semiconductor Composites. Picosecond Dynamics of CdS-Capped Gold Nanoclusters
Abstract
Composite nanoclusters of gold and CdS with core/shell geometry have been synthesized using a chemical precipitation method in aqueous media. These nanoclusters are photoactive and exhibit transient bleaching in the 400−600 nm region when subjected to 355 nm laser pulse excitation. Capping of gold colloids with ultrasmall CdS nanoclusters (particle diameter ∼4 nm) significantly alters the picosecond dynamics of the gold core. The bleaching of the surface plasmon absorption of the gold core is achieved by exciting the CdS shell. The major fraction of the interparticle electron transfer between CdS and Au nanoclusters is completed within the laser pulse duration of 18 ps.
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Cites
Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen
Mie, G. (1908) · Annalen der Physik · doi:10.1002/andp.19083300302 · Cited by 11,537
Perspectives on the Physical Chemistry of Semiconductor Nanocrystals
Alivisatos, A. P. (1996) · The Journal of Physical Chemistry · doi:10.1021/jp9535506 · Cited by 3,595
Cited by
Photophysical, Photochemical and Photocatalytic Aspects of Metal Nanoparticles
Kamat, P. V. (2002) · The Journal of Physical Chemistry B · doi:10.1021/jp0209289 · Cited by 1,924
Self-citationSonochemical Synthesis of SnO2 Nanoparticles and Their Preliminary Study as Li Insertion Electrodes
Zhu, J., Lu, Z., Aruna, S. T., Aurbach, D., & Gedanken, A. (2000) · Chemistry of Materials · doi:10.1021/cm990683l · Cited by 341
Dai, X., Xie, M., Meng, S., Fu, X., & Chen, S. (2014) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2014.04.035 · Cited by 288
Metadata
- Authors
- Kamat, P. V., & Shanghavi, B.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 1997-09-01
- Volume
- 101
- Issue
- 39
- Pages
- 7675-7679
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W2064295842
- Cited by
- 183
- References
- 2
- FWCI
- 2.72
- Type
- journal article
- Language
- en
- Open access
- closed
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