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Adsorption Equilibria of C1to C4Alkanes, CO2, and SF6on Silicalite
Abstract
Adsorption isotherms of methane, ethane, propane, n -butane, isobutane, carbon dioxide, and sulfur hexafluoride were measured gravimetrically on silicalite crystals at temperatures ranging from 3 to 81 °C and at pressures up to 2000 kPa. A virial equation was used to correlate the experimental data and to calculate the isosteric heats of adsorption and the limiting heats of adsorption at zero loading. The adsorption isotherms of isobutane exhibit inflection points at loadings of 4−6 molecules/unit cell in a certain temperature range. This unusual adsorption behavior is attributed to adsorption of isobutane in different locations of the channel system.
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Citations
Cited by
Molecular Simulations of Zeolites: Adsorption, Diffusion, and Shape Selectivity
Smit, B., & Maesen, T. L. M. (2008) · Chemical Reviews · doi:10.1021/cr8002642 · Cited by 829
Babarao, R., Hu, Z., Jiang, J., Chempath, S., & Sandler, S. I. (2007) · Langmuir · doi:10.1021/la062289p · Cited by 408
Palomino, M., Corma, A., Rey, F., & Valencia, S. (2010) · Langmuir · doi:10.1021/la9026656 · Cited by 289
Gas Adsorption Properties of the Chromium-Based Metal Organic Framework MIL-101
Chowdhury, P., Bikkina, C., & Gumma, S. (2009) · The Journal of Physical Chemistry C · doi:10.1021/jp811418r · Cited by 269
(2003) · doi:10.1201/9780203911167.ch22 · Cited by 39
Metadata
- Authors
- Sun, M. S., Shah, D. B., Xu, H. H., & Talu, O.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 1998-02-01
- Volume
- 102
- Issue
- 8
- Pages
- 1466-1473
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W2497261368
- Cited by
- 220
- References
- 0
- FWCI
- 8.18
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Adsorption Equilibria of C1to C4Alkanes, CO2, and SF6on Silicalite. https://app.cochat.ai/papers/10.1021/jp9730196
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- Sun, M. S., Shah, D. B., Xu, H. H., & Talu, O. (1998). Adsorption Equilibria of C1to C4Alkanes, CO2, and SF6on Silicalite. The Journal of Physical Chemistry B. https://doi.org/10.1021/jp9730196
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