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Reducing Graphene Oxide on a Visible-Light BiVO4 Photocatalyst for an Enhanced Photoelectrochemical Water Splitting
Abstract
Bismuth vanadate (BiVO 4 ) is incorporated with reduced graphene oxide (RGO) using a facile single-step photocatalytic reaction to improve its photoresponse in visible light. Remarkable 10-fold enhancement in photoelectrochemical water splitting reaction is observed on BiVO 4 −RGO composite compared with pure BiVO 4 under visible illumination. This improvement is attributed to the longer electron lifetime of excited BiVO 4 as the electrons are injected to RGO instantly at the site of generation, leading to a minimized charge recombination. Improved contact between BiVO 4 particles with transparent conducting electrode using RGO scaffold also contributes to this photoresponse enhancement.
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Cites
Lightcap, I. V., Kosel, T. H., & Kamat, P. V. (2010) · Nano Letters · doi:10.1021/nl9035109 · Cited by 1,044
Cited by
Graphene-based semiconductor photocatalysts
Xiang, Q., Yu, J., & Jaroniec, M. (2012) · Chem. Soc. Rev. · doi:10.1039/c1cs15172j · Cited by 2,730
Advanced Nanoarchitectures for Solar Photocatalytic Applications
Kubacka, A., Fernández-García, M., & Colón, G. (2012) · Chemical Reviews · doi:10.1021/cr100454n · Cited by 2,373
Abe, R. (2010) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2011.02.003 · Cited by 1,223
Zhang, J., Yu, J., Jaroniec, M., & Gong, J. R. (2012) · Nano Letters · doi:10.1021/nl301831h · Cited by 894
Meng, F., Li, J., Cushing, S. K., Zhi, M., & Wu, N. (2013) · Journal of the American Chemical Society · doi:10.1021/ja404851s · Cited by 643
Metadata
- Authors
- Ng, Y. H., Iwase, A., Kudo, A., & Amal, R.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-08-17
- Volume
- 1
- Issue
- 17
- Pages
- 2607-2612
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2050785814
- Cited by
- 869
- References
- 1
- FWCI
- 31.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ng, Y. H., Iwase, A., Kudo, A., & Amal, R. (2010). Reducing Graphene Oxide on a Visible-Light BiVO4 Photocatalyst for an Enhanced Photoelectrochemical Water Splitting. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/jz100978u
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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