The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
The Raman Spectrum of the CH3NH3PbI3 Hybrid Perovskite: Interplay of Theory and Experiment
Abstract
We report the low-frequency resonant Raman spectrum of methylammonium lead-iodide, a prototypical perovskite for solar cells applications, on mesoporous Al2O3. The measured spectrum assignment is assisted by DFT simulations of the Raman spectra of suitable periodic and model systems. The bands at 62 and 94 cm(-1) are assigned respectively to the bending and to the stretching of the Pb-I bonds, and are thus diagnostic modes of the inorganic cage. We also assign the librations of the organic cations at 119 and 154 cm(-1). The broad, unstructured 200-400 cm(-1) features are assigned to the torsional mode of the methylammonium cations, which we propose as a marker of the orientational disorder of the material. Our study provides the basis to interpret the Raman spectra of organohalide perovskites, which may allow one to further understand the properties of this important class of materials in relation to their full exploitation in solar cells.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
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Cited by
Charge-Carrier Dynamics in Organic-Inorganic Metal Halide Perovskites
Herz, L. M. (2016) · Annual Review of Physical Chemistry · doi:10.1146/annurev-physchem-040215-112222 · Cited by 819
Lead iodide perovskite light-emitting field-effect transistor
Chin, X. Y., Cortecchia, D., Yin, J., Bruno, A., & Soci, C. (2015) · Nature Communications · doi:10.1038/ncomms8383 · Cited by 767
Tuning the Light Emission Properties by Band Gap Engineering in Hybrid Lead Halide Perovskite
D’Innocenzo, V., Srimath Kandada, A. R., De Bastiani, M., Gandini, M., & Petrozza, A. (2014) · Journal of the American Chemical Society · doi:10.1021/ja511198f · Cited by 623
Self-citationZhu, X.-Y., & Podzorov, V. (2015) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.5b02462 · Cited by 608
Jodlowski, A. D., Roldán-Carmona, C., Grancini, G., Salado, M., Ralaiarisoa, M., Ahmad, S., Koch, N., Camacho, L., de Miguel, G., & Nazeeruddin, M. K. (2017) · Nature Energy · doi:10.1038/s41560-017-0054-3 · Cited by 533
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Metadata
- Authors
- Quarti, C., Grancini, G., Mosconi, E., Bruno, P., Ball, J. M., Lee, M. M., Snaith, H. J., Petrozza, A., & De Angelis, F.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-12-26
- Volume
- 5
- Issue
- 2
- Pages
- 279-284
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2044423188
- Cited by
- 654
- References
- 1
- FWCI
- 32.55
- Type
- journal article
- Language
- en
- Open access
- closed
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- Quarti, C., Grancini, G., Mosconi, E., Bruno, P., Ball, J. M., Lee, M. M., Snaith, H. J., Petrozza, A., & De Angelis, F. (2014). The Raman Spectrum of the CH3NH3PbI3 Hybrid Perovskite: Interplay of Theory and Experiment. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/jz402589q
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