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Activity–Stability Trends for the Oxygen Evolution Reaction on Monometallic Oxides in Acidic Environments
Abstract
In the present study, we used a surface-science approach to establish a functional link between activity and stability of monometallic oxides during the OER in acidic media. We found that the most active oxides (Au ≪ Pt < Ir < Ru ≪ Os) are, in fact, the least stable (Au ≫ Pt > Ir > Ru ≫ Os) materials. We suggest that the relationships between stability and activity are controlled by both the nobility of oxides as well as by the density of surface defects. This functionality is governed by the nature of metal cations and the potential transformation of a stable metal cation with a valence state of n = +4 to unstable metal cation with n > +4. A practical consequence of such a close relationship between activity and stability is that the best materials for the OER should balance stability and activity in such a way that the dissolution rate is neither too fast nor too slow.
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Cites
Enhancing Hydrogen Evolution Activity in Water Splitting by Tailoring Li + -Ni(OH) 2 -Pt Interfaces
Subbaraman, R., Tripkovic, D., Strmcnik, D., Chang, K.-C., Uchimura, M., Paulikas, A. P., Stamenkovic, V., & Markovic, N. M. (2011) · Science · doi:10.1126/science.1211934 · Cited by 3,135
Self-citationImproving the hydrogen oxidation reaction rate by promotion of hydroxyl adsorption
Strmcnik, D., Uchimura, M., Wang, C., Subbaraman, R., Danilovic, N., van der Vliet, D., Paulikas, A. P., Stamenkovic, V. R., & Markovic, N. M. (2013) · Nature Chemistry · doi:10.1038/nchem.1574 · Cited by 1,426
Self-citation
Cited by
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Shinagawa, T., Garcia-Esparza, A. T., & Takanabe, K. (2015) · Scientific Reports · doi:10.1038/srep13801 · Cited by 3,287
Chen, F.-Y., Wu, Z.-Y., Adler, Z., & Wang, H. (2021) · Joule · doi:10.1016/j.joule.2021.05.005 · Cited by 1,284
Reier, T., Nong, H. N., Teschner, D., Schlögl, R., & Strasser, P. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201601275 · Cited by 1,253
Recent Progress on Multimetal Oxide Catalysts for the Oxygen Evolution Reaction
Kim, J. S., Kim, B., Kim, H., & Kang, K. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702774 · Cited by 940
Metadata
- Authors
- Danilovic, N., Subbaraman, R., Chang, K.-C., Chang, S. H., Kang, Y. J., Snyder, J., Paulikas, A. P., Strmcnik, D., Kim, Y.-T., Myers, D., Stamenkovic, V. R., & Markovic, N. M.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-07-07
- Volume
- 5
- Issue
- 14
- Pages
- 2474-2478
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2331528766
- Cited by
- 758
- References
- 2
- FWCI
- 11.79
- Type
- journal article
- Language
- en
- Open access
- closed
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- Danilovic, N., Subbaraman, R., Chang, K.-C., Chang, S. H., Kang, Y. J., Snyder, J., Paulikas, A. P., Strmcnik, D., Kim, Y.-T., Myers, D., Stamenkovic, V. R., & Markovic, N. M. (2014). Activity–Stability Trends for the Oxygen Evolution Reaction on Monometallic Oxides in Acidic Environments. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/jz501061n
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