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Ultra-Low Thermal Conductivity in Organic–Inorganic Hybrid Perovskite CH3NH3PbI3
Open accessAbstract
We report on the temperature dependence of thermal conductivity of single crystalline and polycrystalline organometallic perovskite CH3NH3PbI3. The comparable absolute values and temperature dependence of the two samples' morphologies indicate the minor role of the grain boundaries on the heat transport. Theoretical modeling demonstrates the importance of the resonant scattering in both specimens. The interaction between phonon waves and rotational degrees of freedom of CH3NH3(+) sublattice emerges as the dominant mechanism for attenuation of heat transport and for ultralow thermal conductivity of 0.5 W/(Km) at room temperature.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Resonant bonding leads to low lattice thermal conductivity
Lee, S., Esfarjani, K., Luo, T., Zhou, J., Tian, Z., & Chen, G. (2014) · Nature Communications · doi:10.1038/ncomms4525 · Cited by 679
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Leguy, A. M. A., Goñi, A. R., Frost, J. M., Skelton, J., Brivio, F., Rodríguez-Martínez, X., Weber, O. J., Pallipurath, A., Alonso, M. I., Campoy-Quiles, M., et al. (2016) · Physical Chemistry Chemical Physics · doi:10.1039/c6cp03474h · Cited by 459
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Metadata
- Authors
- Pisoni, A., Jaćimović, J., Barišić, O. S., Spina, M., Gaál, R., Forró, L., & Horváth, E.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-07-08
- Volume
- 5
- Issue
- 14
- Pages
- 2488-2492
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2050079556
- Cited by
- 521
- References
- 2
- FWCI
- 19.66
- Type
- journal article
- Language
- en
- Open access
- green
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- Pisoni, A., Jaćimović, J., Barišić, O. S., Spina, M., Gaál, R., Forró, L., & Horváth, E. (2014). Ultra-Low Thermal Conductivity in Organic–Inorganic Hybrid Perovskite CH3NH3PbI3. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/jz5012109
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