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Interaction of Silane Coupling Agents with Cellulose
Abstract
The adsorption of several prehydrolyzed alkoxysilanes onto the surface of cellulosic fibers in ethanol/water mixtures has been studied quantitatively. The corresponding isotherms show the formation of a monolayer followed by further adsorption. The nature of the fourth substituent on the silane plays a specific role on the features of this association. Whereas at room temperature only dispersive and polar attractive interactions occur, heating above 100 °C produces condensation reactions resulting in covalent bonding between the substrate and the silane forming the monolayer. As a result of this investigation, the possibility of calling upon this surface modification in order to compatibilize cellulosic fibers with polyolefinic matrixes for the elaboration of composite materials seems to be a promising strategy.
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Citations
Cited by
Cellulosic nanocomposites: a review
(2008) · BioResources · doi:10.15376/biores.3.3.929-980 · Cited by 901
Jagadeesh, P., Puttegowda, M., Mavinkere Rangappa, S., & Siengchin, S. (2021) · Polymer Composites · doi:10.1002/pc.26312 · Cited by 281
Mechanical and thermal conductivity properties of hemp fiber reinforced polyurethane composites
Sair, S., Oushabi, A., Kammouni, A., Tanane, O., Abboud, Y., & El Bouari, A. (2018) · Case Studies in Construction Materials · doi:10.1016/j.cscm.2018.02.001 · Cited by 174
Surface esterification of cellulose fibers: Characterization by DRIFT and contact angle measurements
Pasquini, D., Belgacem, M. N., Gandini, A., & Curvelo, A. A. D. S. (2006) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2005.07.074 · Cited by 134
Self-citationLy, B., Thielemans, W., Dufresne, A., Chaussy, D., & Belgacem, M. N. (2008) · Composites Science and Technology · doi:10.1016/j.compscitech.2008.07.018 · Cited by 129
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Metadata
- Authors
- Abdelmouleh, M., Boufi, S., ben Salah, A., Belgacem, M. N., & Gandini, A.
- Venue
- Langmuir
- Publisher
- American Chemical Society (ACS)
- Published
- 2002-03-19
- Volume
- 18
- Issue
- 8
- Pages
- 3203-3208
- ISSN
- 0743-7463 (ISSN-L)
- 1520-5827
- OpenAlex
- W2028414274
- Cited by
- 320
- References
- 0
- FWCI
- 20.65
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
