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Glucose-Responsive Polyelectrolyte Capsules
Abstract
Phenylboronic acids are known to form covalent complexes with polyol compounds such as glucose. A novel polyelectrolyte, containing phenylboronic acid as a glucose-sensitive moiety, has been synthesized and used for the fabrication of glucose-sensitive hollow polyelectrolyte capsules using the layer-by-layer technique. The response to glucose was observed as a rather fast dissolution of the capsules when brought into contact with a glucose-containing medium. These polyelectrolyte capsules are the first polyelectrolyte capsules able to respond to a stimulus that can be provided by the human body (i.e., an increase in glucose concentration). Therefore, the concept we present has promising applications in the biomedical field for the controlled delivery of insulin.
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Citations
Cited by
Ariga, K., Hill, J. P., & Ji, Q. (2007) · Physical Chemistry Chemical Physics · doi:10.1039/b700410a · Cited by 1,256
Stimulus-responsive hydrogels: theory, modern advances, and applications
Koetting, M. C., Peters, J. T., Steichen, S. D., & Peppas, N. A. (2015) · Materials Science and Engineering: R: Reports · doi:10.1016/j.mser.2015.04.001 · Cited by 1,191
Motornov, M., Roiter, Y., Tokarev, I., & Minko, S. (2010) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2009.10.004 · Cited by 773
Challenges and breakthroughs in recent research on self-assembly
Ariga, K., Hill, J. P., Lee, M. V., Vinu, A., Charvet, R., & Acharya, S. (2008) · Science and Technology of Advanced Materials · doi:10.1088/1468-6996/9/1/014109 · Cited by 759
Stimuli-responsive LbL capsules and nanoshells for drug delivery
Delcea, M., Möhwald, H., & Skirtach, A. G. (2011) · Advanced Drug Delivery Reviews · doi:10.1016/j.addr.2011.03.010 · Cited by 685
Metadata
- Authors
- De Geest, B. G., Jonas, A. M., Demeester, J., & De Smedt, S. C.
- Venue
- Langmuir
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-04-29
- Volume
- 22
- Issue
- 11
- Pages
- 5070-5074
- ISSN
- 0743-7463 (ISSN-L)
- 1520-5827
- OpenAlex
- W2086727955
- Cited by
- 193
- References
- 0
- FWCI
- 6.44
- Type
- journal article
- Language
- en
- Open access
- closed
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- De Geest, B. G., Jonas, A. M., Demeester, J., & De Smedt, S. C. (2006). Glucose-Responsive Polyelectrolyte Capsules. Langmuir. https://doi.org/10.1021/la053368o
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