The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Metal–Organic Frameworks for Removal of Xe and Kr from Nuclear Fuel Reprocessing Plants
Abstract
Removal of xenon (Xe) and krypton (Kr) from process off-gases containing 400 ppm Xe, 40 ppm Kr, 78% N(2), 21% O(2), 0.9% Ar, 0.03% CO(2), and so forth using adsorption was demonstrated for the first time. Two well-known metal-organic frameworks (MOFs), HKUST-1 and Ni/DOBDC, which both have unsaturated metal centers but different pore morphologies, were selected as novel adsorbents. Results of an activated carbon were also included for comparison. The Ni/DOBDC has higher Xe/Kr selectivities than those of the activated carbon and the HKUST-1. In addition, results show that the Ni/DOBDC and HKUST-1 can adsorb substantial amounts of Xe and Kr even when they are mixed in air. Moreover, the Ni/DOBDC can successfully separate 400 ppm Xe from 40 ppm Kr and air containing O(2), N(2), and CO(2) with a Xe/Ke selectivity of 7.3 as indicated by our breakthrough results. This shows a promising future for MOFs in radioactive nuclide separations from spent fuels.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Millward, A. R., & Yaghi, O. M. (2005) · Journal of the American Chemical Society · doi:10.1021/ja0570032 · Cited by 2,876
Industrial Gas Handbook: Gas Separation and Purification
Kerry, F. G. (2007) · doi:10.1201/9781420008265 · Cited by 297
Cited by
Metal–Organic Frameworks for Separation
Zhao, X., Wang, Y., Li, D., Bu, X., & Feng, P. (2018) · Advanced Materials · doi:10.1002/adma.201705189 · Cited by 1,305
CO2 Capture and Separations Using MOFs: Computational and Experimental Studies
Yu, J., Xie, L.-H., Li, J.-R., Ma, Y., Seminario, J. M., & Balbuena, P. B. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00626 · Cited by 1,047
Metal–Organic Frameworks for Air Purification of Toxic Chemicals
DeCoste, J. B., & Peterson, G. W. (2014) · Chemical Reviews · doi:10.1021/cr4006473 · Cited by 958
Sensing and capture of toxic and hazardous gases and vapors by metal–organic frameworks
Wang, H., Lustig, W. P., & Li, J. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00885f · Cited by 695
Separation of rare gases and chiral molecules by selective binding in porous organic cages
Chen, L., Reiss, P. S., Chong, S. Y., Holden, D., Jelfs, K. E., Hasell, T., Little, M. A., Kewley, A., Briggs, M. E., Stephenson, A., et al. (2014) · Nature Materials · doi:10.1038/nmat4035 · Cited by 666
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Metadata
- Authors
- Liu, J., Thallapally, P. K., & Strachan, D.
- Venue
- Langmuir
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-07-26
- Volume
- 28
- Issue
- 31
- Pages
- 11584-11589
- ISSN
- 0743-7463 (ISSN-L)
- 1520-5827
- OpenAlex
- W2020535926
- Cited by
- 216
- References
- 3
- FWCI
- 7.17
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, J., Thallapally, P. K., & Strachan, D. (2012). Metal–Organic Frameworks for Removal of Xe and Kr from Nuclear Fuel Reprocessing Plants. Langmuir. https://doi.org/10.1021/la301870n
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