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Formation and Stability of Multilayers of Polyelectrolytes
Open accessAbstract
Sequential addition of anionic and cationic polyelectrolytes may lead to the formation of multilayers at a solid surface. The buildup of such multilayers is characterized by a stepwise increase of the adsorbed amount and layer thickness and by alternating highly positive and highly negative values for the ζ-potential. The prime variables which determine the stability of these structures are the polymer charge and the ionic strength. Very stable multilayers are formed when both polymers are highly charged and when the ionic strength is low. For weakly stable multilayers complexation at the surface may first occur, followed by desorption of the complexes. For strongly charged polyelectrolytes the charge stoichiometry, which is not always 1:1, seems to be unique for each pair of polyelectrolytes; no influence of the substrate, of the pH, or of the ionic strength could be observed.
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Cited by
Fuzzy Nanoassemblies: Toward Layered Polymeric Multicomposites
Decher, G. (1997) · Science · doi:10.1126/science.277.5330.1232 · Cited by 10,054
Technology-driven layer-by-layer assembly of nanofilms
Richardson, J. J., Björnmalm, M., & Caruso, F. (2015) · Science · doi:10.1126/science.aaa2491 · Cited by 1,641
Ariga, K., Hill, J. P., & Ji, Q. (2007) · Physical Chemistry Chemical Physics · doi:10.1039/b700410a · Cited by 1,256
Yoo, D., Shiratori, S. S., & Rubner, M. F. (1998) · Macromolecules · doi:10.1021/ma9800360 · Cited by 867
Layer-by-layer self assembly of polyelectrolytes on colloidal particles
Sukhorukov, G. B., Donath, E., Lichtenfeld, H., Knippel, E., Knippel, M., Budde, A., & Möhwald, H. (1998) · Colloids and Surfaces A: Physicochemical and Engineering Aspects · doi:10.1016/s0927-7757(98)00213-1 · Cited by 830
Metadata
- Authors
- Hoogeveen, N. G., Cohen Stuart, M. A., Fleer, G. J., & Böhmer, M. R.
- Venue
- Langmuir
- Publisher
- American Chemical Society (ACS)
- Published
- 1996-01-01
- Volume
- 12
- Issue
- 15
- Pages
- 3675-3681
- ISSN
- 0743-7463 (ISSN-L)
- 1520-5827
- OpenAlex
- W2041552752
- Cited by
- 412
- References
- 0
- FWCI
- 6.65
- Type
- journal article
- Language
- en
- Open access
- green
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- Hoogeveen, N. G., Cohen Stuart, M. A., Fleer, G. J., & Böhmer, M. R. (1996). Formation and Stability of Multilayers of Polyelectrolytes. Langmuir. https://doi.org/10.1021/la951574y
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