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Multilayer Nanoreactors for Metallic and Semiconducting Particles
Abstract
Multilayer thin films of sequentially adsorbed polyelectrolytes were utilized as nanoreactors for both metallic (Ag) and semiconductor nanoparticles (PbS). Polyelectrolyte multilayers with a controlled content of free carboxylic acid binding groups were fabricated with weak polyelectrolytes via suitable pH adjustments of the processing solutions. These groups were then used to bind various inorganic ions that were subsequently converted into nanoparticles. Spatial control (at the nanoscale) over the growth of the nanoparticles was achieved via the use of multilayer heterostructures that also contain bilayer blocks that are not able to bind inorganic ions. These “nonbinding” bilayers were fabricated from strong polyacids such as poly(styrene sulfonic acid). TEM imaging of the nanoparticles within the multilayer thin films indicates that the polycation and polyanion layers of these films are highly interpenetrated.
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Cited by
Banerjee, I., Pangule, R. C., & Kane, R. S. (2011) · Advanced Materials · doi:10.1002/adma.201001215 · Cited by 2,749
Self-citationForm and Function in Multilayer Assembly: New Applications at the Nanoscale
Hammond, P. T. (2004) · Advanced Materials · doi:10.1002/adma.200400760 · Cited by 1,251
Molecular basis for the explanation of the exponential growth of polyelectrolyte multilayers
Picart, C., Mutterer, J., Richert, L., Luo, Y., Prestwich, G. D., Schaaf, P., Voegel, J.-C., & Lavalle, P. (2002) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.202486099 · Cited by 904
Silver bromide nanoparticle/polymer composites: dual action tunable antimicrobial materials
Sambhy, V., MacBride, M. M., Peterson, B. R., & Sen, A. (2006) · Journal of the American Chemical Society · doi:10.1021/ja061442z · Cited by 748
Lee, D., Cohen, R. E., & Rubner, M. F. (2005) · Langmuir · doi:10.1021/la0513306 · Cited by 484
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Metadata
- Authors
- Joly, S., Kane, R., Radzilowski, L., Wang, T., Wu, A., Cohen, R. E., Thomas, E. L., & Rubner, M. F.
- Venue
- Langmuir
- Publisher
- American Chemical Society (ACS)
- Published
- 1999-12-28
- Volume
- 16
- Issue
- 3
- Pages
- 1354-1359
- ISSN
- 0743-7463 (ISSN-L)
- 1520-5827
- OpenAlex
- W1966172365
- Cited by
- 299
- References
- 0
- FWCI
- 12.23
- Type
- journal article
- Language
- en
- Open access
- closed
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- Joly, S., Kane, R., Radzilowski, L., Wang, T., Wu, A., Cohen, R. E., Thomas, E. L., & Rubner, M. F. (2000). Multilayer Nanoreactors for Metallic and Semiconducting Particles. Langmuir. https://doi.org/10.1021/la991089t
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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