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Janus Micelles
Open accessAbstract
A novel strategy to synthesize amphiphilic surface-compartmentalized nanoparticles based on linear ABC triblock copolymers is presented. These so-called Janus micelles consist of a cross-linked core and a corona with a “northern” and a “southern” hemisphere. Selectively cross-linking spherical domains of the polybutadiene middle block in a well-ordered bulk morphology of a polystyrene- block -polybutadiene- block -poly(methyl methacrylate) triblock copolymer (SBM) leads to the conservation of the compartmentalization of the outer blocks after dissolution of the material. Multi-angle laser light scattering gel permeation chromatography, fluorescence correlation spectroscopy, small-angle neutron scattering, and static and dynamic light scattering, as well as scanning force microscopy, indicate the existence of an equilibrium between molecularly dissolved Janus micelles (unimers) and aggregates (multimers), so-called supermicelles.
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Citations
Cited by
Janus Particles: Synthesis, Self-Assembly, Physical Properties, and Applications
Walther, A., & Müller, A. H. E. (2013) · Chemical Reviews · doi:10.1021/cr300089t · Cited by 1,769
Self-citationBlanazs, A., Armes, S. P., & Ryan, A. J. (2009) · Macromolecular Rapid Communications · doi:10.1002/marc.200800713 · Cited by 1,500
Block Copolymers: Past Successes and Future Challenges
Lodge, T. P. (2003) · Macromolecular Chemistry and Physics · doi:10.1002/macp.200290073 · Cited by 567
Water-Soluble Stimuli-Responsive Vesicles from Peptide-Based Diblock Copolymers
Chécot, F., Lecommandoux, S., Gnanou, Y., & Klok, H.-A. (2002) · Angewandte Chemie International Edition · doi:10.1002/1521-3773(20020415)41:8<1339::aid-anie1339>3.0.co;2-n · Cited by 384
Self-Assembly of Copolymer Micelles: Higher-Level Assembly for Constructing Hierarchical Structure
Lu, Y., Lin, J., Wang, L., Zhang, L., & Cai, C. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00774 · Cited by 281
Metadata
- Authors
- Erhardt, R., Böker, A., Zettl, H., Kaya, H., Pyckhout-Hintzen, W., Krausch, G., Abetz, V., & Müller, A. H. E.
- Venue
- Macromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2001-01-17
- Volume
- 34
- Issue
- 4
- Pages
- 1069-1075
- ISSN
- 0024-9297 (ISSN-L)
- 1520-5835
- OpenAlex
- W4236200760
- Cited by
- 396
- References
- 0
- FWCI
- 11.23
- Type
- journal article
- Language
- en
- Open access
- green
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- Erhardt, R., Böker, A., Zettl, H., Kaya, H., Pyckhout-Hintzen, W., Krausch, G., Abetz, V., & Müller, A. H. E. (2001). Janus Micelles. Macromolecules. https://doi.org/10.1021/ma000670p
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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