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Suspensions of Silica Particles Grafted with Concentrated Polymer Brush: A New Family of Colloidal Crystals
Abstract
A colloidal crystal was newly identified for a liquid suspension of the hybrid particles having a spherical silica core and a shell of well-defined poly(methyl methacrylate) “concentrated brush”. With increasing particle concentration, the suspension progressed from a (disordered) fluid to a fully crystallized system, going through a narrow crystal/fluid coexisting regime. The crystal had a face-centered cubic structure with a surprisingly large nearest-neighbor interparticle distance, suggesting that the graft chains, highly extended due to the “concentrated brush effect”, exerted a long-range steric interaction. This type of colloidal crystal is new with respect to the origin of long-range interparticle potential and the controllability of many of the system parameters.
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Cited by
Barbey, R., Lavanant, L., Paripovic, D., Schüwer, N., Sugnaux, C., Tugulu, S., & Klok, H.-A. (2009) · Chemical Reviews · doi:10.1021/cr900045a · Cited by 1,753
Zoppe, J. O., Ataman, N. C., Mocny, P., Wang, J., Moraes, J., & Klok, H.-A. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00314 · Cited by 1,046
Nanocomposites with Polymer Grafted Nanoparticles
Kumar, S. K., Jouault, N., Benicewicz, B., & Neely, T. (2013) · Macromolecules · doi:10.1021/ma4001385 · Cited by 772
Metadata
- Authors
- Ohno, K., Morinaga, T., Takeno, S., Tsujii, Y., & Fukuda, T.
- Venue
- Macromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-12-31
- Volume
- 39
- Issue
- 3
- Pages
- 1245-1249
- ISSN
- 0024-9297 (ISSN-L)
- 1520-5835
- OpenAlex
- W2076957588
- Cited by
- 163
- References
- 0
- FWCI
- 3.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Suspensions of Silica Particles Grafted with Concentrated Polymer Brush: A New Family of Colloidal Crystals. https://app.cochat.ai/papers/10.1021/ma0521708
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- Ohno, K., Morinaga, T., Takeno, S., Tsujii, Y., & Fukuda, T. (2006). Suspensions of Silica Particles Grafted with Concentrated Polymer Brush: A New Family of Colloidal Crystals. Macromolecules. https://doi.org/10.1021/ma0521708
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
