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Distribution of Nanoparticles in Lamellar Domains of Block Copolymers
Abstract
Polystyrene-coated gold nanoparticles (molecular weight ( M n ) of PS ∼1300 g/mol, average particle diameter d (core + shell) ∼ 9.2 ± 2.2 nm, corresponding to a high areal chain density of PS) are incorporated into symmetric poly(styrene- b -2 vinylpyridine) diblock copolymers with total M n ∼ 60 000−380 000 g/mol at volume fractions of 0.07−0.32. For all M n of diblock copolymers and particle filling fractions examined, particles are centralized in the PS domains with Gaussian distribution profiles. The distribution width generally decreases as the PS domain size decreases or as the particle weight fraction increases. These observations are discussed in terms of the relative entropic contributions of the polymer chains and particles.
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Beaumont, C., Jamieson, R. A., Nguyen, M. H., & Lee, B. (2001) · Nature · doi:10.1038/414738a · Cited by 1,632
Cited by
Toward functional nanocomposites: taking the best of nanoparticles, polymers, and small molecules
Kao, J., Thorkelsson, K., Bai, P., Rancatore, B. J., & Xu, T. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35375j · Cited by 386
Walther, A., Matussek, K., & Müller, A. H. E. (2008) · ACS Nano · doi:10.1021/nn800108y · Cited by 310
Yetisen, A. K., Butt, H., Volpatti, L. R., Pavlichenko, I., Humar, M., Kwok, S. J. J., Koo, H., Kim, K. S., Naydenova, I., Khademhosseini, A., et al. (2016) · Biotechnology Advances · doi:10.1016/j.biotechadv.2015.10.005 · Cited by 192
Metadata
- Authors
- Chiu, J. J., Kim, B. J., Yi, G.-R., Bang, J., Kramer, E. J., & Pine, D. J.
- Venue
- Macromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-03-21
- Volume
- 40
- Issue
- 9
- Pages
- 3361-3365
- ISSN
- 0024-9297 (ISSN-L)
- 1520-5835
- OpenAlex
- W2079536149
- Cited by
- 159
- References
- 1
- FWCI
- 4.57
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chiu, J. J., Kim, B. J., Yi, G.-R., Bang, J., Kramer, E. J., & Pine, D. J. (2007). Distribution of Nanoparticles in Lamellar Domains of Block Copolymers. Macromolecules. https://doi.org/10.1021/ma061503d
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