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SCFT Study of Nonfrustrated ABC Triblock Copolymer Melts
Abstract
The phase behavior of ABC triblock copolymer melts is studied by self-consistent-field theory (SCFT). We focus on “nonfrustrated” triblocks, in which the Flory−Huggins interaction parameter χ AC between the end blocks is significantly larger than that between the middle and either end block, i.e., χ AC ≫ χ AB ∼ χ BC . Such systems tend to form ordered structures with no AC interface. Complete phase triangles at fixed values of the products χ ij N are presented for a model with χ AB = χ BC ≪ χ AC and for a model with parameters chosen to represent poly(isoprene- b -styrene- b -ethylene oxide) copolymers that have recently been studied experimentally. Particular attention is paid to the structure of the orthorhombic O 70 network phase and the reasons for its existence as well as to the sensitivity of the predicted phase behavior to changes in the χ parameters.
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Citations
Cited by
Orilall, M. C., & Wiesner, U. (2011) · Chem. Soc. Rev. · doi:10.1039/c0cs00034e · Cited by 520
Block copolymer electrolytes for rechargeable lithium batteries
Young, W., Kuan, W., & Epps (2014) · Journal of Polymer Science Part B: Polymer Physics · doi:10.1002/polb.23404 · Cited by 417
Discovering ordered phases of block copolymers: New results from a generic fourier-space approach
Guo, Z., Zhang, G., Qiu, F., Zhang, H., Yang, Y., & Shi, A.-C. (2008) · Physical Review Letters · doi:10.1103/physrevlett.101.028301 · Cited by 150
Metadata
- Authors
- Tyler, C. A., Qin, J., Bates, F. S., & Morse, D. C.
- Venue
- Macromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-06-01
- Volume
- 40
- Issue
- 13
- Pages
- 4654-4668
- ISSN
- 0024-9297 (ISSN-L)
- 1520-5835
- OpenAlex
- W2154993942
- Cited by
- 187
- References
- 0
- FWCI
- 6.95
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tyler, C. A., Qin, J., Bates, F. S., & Morse, D. C. (2007). SCFT Study of Nonfrustrated ABC Triblock Copolymer Melts. Macromolecules. https://doi.org/10.1021/ma062778w
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