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Mechanical Reinforcement in Polymer Melts Filled with Polymer Grafted Nanoparticles
Abstract
We critically leverage the fact that polymer grafted nanoparticles behave akin to block copolymers to systematically vary nanoparticle dispersion and critically examine its role on the mechanical reinforcement in liquid-polymer-based nanocomposites. The nanoparticles are noncontacting, and we perform rheological measurements 80K above the polymer’s glass transition temperature. Our rheology results unequivocally show that reinforcement is maximized by the formation of a transient, but long-lived, percolating polymer–particle network with the particles serving as the network junctions.
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Cites
Effect of silica nanoparticles on the local segmental dynamics in poly (vinyl acetate)
Bogoslovov, R. B., Roland, C. M., Ellis, A. R., Randall, A. M., & Robertson, C. G. (2008) · Macromolecules · doi:10.1021/ma702372a · Cited by 176
Cited by
Hui, C. M., Pietrasik, J., Schmitt, M., Mahoney, C., Choi, J., Bockstaller, M. R., & Matyjaszewski, K. (2014) · Chemistry of Materials · doi:10.1021/cm4023634 · Cited by 367
Topologically Induced Heterogeneity in Gradient Copolymer Brush Particle Materials
Zhao, Y., Wang, Z., Yu, C., Wu, H., Olszewski, M., Yin, R., Zhai, Y., Liu, T., Coronado, A., Matyjaszewski, K., et al. (2022) · Macromolecules · doi:10.1021/acs.macromol.2c01131 · Cited by 20
Metadata
- Authors
- Moll, J. F., Akcora, P., Rungta, A., Gong, S., Colby, R. H., Benicewicz, B. C., & Kumar, S. K.
- Venue
- Macromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-08-24
- Volume
- 44
- Issue
- 18
- Pages
- 7473-7477
- ISSN
- 0024-9297 (ISSN-L)
- 1520-5835
- OpenAlex
- W2324975076
- Cited by
- 216
- References
- 1
- FWCI
- 8.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- Moll, J. F., Akcora, P., Rungta, A., Gong, S., Colby, R. H., Benicewicz, B. C., & Kumar, S. K. (2011). Mechanical Reinforcement in Polymer Melts Filled with Polymer Grafted Nanoparticles. Macromolecules. https://doi.org/10.1021/ma201200m
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