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Diketopyrrolopyrrole-Based Semiconducting Polymer for Photovoltaic Device with Photocurrent Response Wavelengths up to 1.1 μm
Abstract
A highly effective photovoltaic polymer with near-infrared response, poly{ N -[1-(2-ethylhexyl)-3-ethylheptanyl]-dithieno[3,2- b:2′,3′- d ]pyrrole - 3,6-dithien-2-yl-2,5-dibutylpyrrolo[3,4- c ]pyrrole-1,4-dione-5′,5′′-diyl} {PDTP-DTDPP(Bu)}, was synthesized. The polymer has high molecular weight, good solubility, and a broad absorption spectrum in the range of 500−1100 nm. Field effect transistor charge mobility of PDTP-DTDPP(Bu) arrived 0.05 cm 2 V −1 s −1 . Bulk heterojunction type polymer solar cells based on PDTP-DTDPP(Bu) and PC 70 BM have broad photocurrent response wavelength range from 300 nm to 1.1 μm. High short-circuit current (14.87 mA/cm 2 ) and power conversion efficiency (2.71%) were achieved, which is a significant advance for efficient photovoltaic polymers that respond to the whole range of the solar spectrum.
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Citations
Cites
Conjugated Polymer-Based Organic Solar Cells
Günes, S., Neugebauer, H., & Sariciftci, N. S. (2007) · Chemical Reviews · doi:10.1021/cr050149z · Cited by 6,279
Cited by
Efficient Tandem and Triple-Junction Polymer Solar Cells
Li, W., Furlan, A., Hendriks, K. H., Wienk, M. M., & Janssen, R. A. J. (2013) · Journal of the American Chemical Society · doi:10.1021/ja401434x · Cited by 507
Design of Diketopyrrolopyrrole (DPP)‐Based Small Molecules for Organic‐Solar‐Cell Applications
Tang, A., Zhan, C., Yao, J., & Zhou, E. (2017) · Advanced Materials · doi:10.1002/adma.201600013 · Cited by 348
Self-citationChochos, C. L., & Choulis, S. A. (2011) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2011.04.003 · Cited by 340
A near-infrared non-fullerene electron acceptor for high performance polymer solar cells
Li, Y., Zhong, L., Gautam, B., Bin, H.-J., Lin, J.-D., Wu, F.-P., Zhang, Z., Jiang, Z.-Q., Zhang, Z.-G., Gundogdu, K., et al. (2017) · Energy & Environmental Science · doi:10.1039/c7ee00844a · Cited by 284
New conjugated polymers for plastic solar cells
Gendron, D., & Leclerc, M. (2011) · Energy & Environmental Science · doi:10.1039/c1ee01072g · Cited by 264
Metadata
- Authors
- Zhou, E., Wei, Q., Yamakawa, S., Zhang, Y., Tajima, K., Yang, C., & Hashimoto, K.
- Venue
- Macromolecules
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-12-28
- Volume
- 43
- Issue
- 2
- Pages
- 821-826
- ISSN
- 0024-9297 (ISSN-L)
- 1520-5835
- OpenAlex
- W2027824574
- Cited by
- 185
- References
- 1
- FWCI
- 24.02
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Zhou, E., Wei, Q., Yamakawa, S., Zhang, Y., Tajima, K., Yang, C., & Hashimoto, K. (2010). Diketopyrrolopyrrole-Based Semiconducting Polymer for Photovoltaic Device with Photocurrent Response Wavelengths up to 1.1 μm. Macromolecules. https://doi.org/10.1021/ma902398q
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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