Cited by 150Polymer crystallization and propertiesMaterial Dynamics and PropertiesMicrostructure and mechanical properties

The DOI matches its Crossref record; 21 of the 21 references it cites were found in a registry or an index.

Plastic Deformation Mechanisms of Semicrystalline and Amorphous Polymers

Jabbari-Farouji, Sara, Rottler, Joerg, Lame, Olivier, Makke, Ali, Perez, Michel, Barrat, Jean-Louis·2015·ACS Macro Letters

Abstract

We use large-scale molecular dynamics simulations to investigate plastic deformation of semicrystalline polymers with randomly nucleated crystallites. The strain-softening regime is dominated by deformation of crystallites via reorientation of chain-folded lamellae toward the tensile axis, fragmentation of largest crystalline domains, and a partial loss of crystallinity. The strain-hardening regime coincides with unfolding of chains and recrystallization as a result of strain-induced chain alignment. These observed deformation mechanisms are consistent with experimental findings. We compare the tensile behavior of semicrystalline polymers with their amorphous counterparts at temperatures above and below the glass transition temperature.

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Crossref · 10.1021/mz500754b

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Research works printed but not linked: 3

  1. Young R. J., 1976, Philos. Mag., 30, 86
  2. Wang Y., 2013, Macromolecules, 46, 518522
  3. Jiang Z., 2010, Macromolecules, 43, 472732

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Metadata

Authors
Jabbari-Farouji, S., Rottler, J., Lame, O., Makke, A., Perez, M., & Barrat, J.-L.
Affiliations
  • Université Grenoble Alpes, UJF Liphy, F38041 Grenoble, France
  • Department of Physics and Astronomy, The University of British Columbia, 6224 Agricultural Road, Vancouver, British Columbia V6T 1Z1, Canada
  • Centre National de la Recherche Scientifique (FR)
  • Université Joseph Fourier (FR)
Venue
ACS Macro Letters
Published
2015-01-14
Volume
4
Issue
2
Pages
147-150
ISSN
2161-1653 (ISSN-L)
OpenAlex
W2314025514
Cited by
147
References
21
Citations by year
2026: 19 · 2025: 11 · 2024: 19 · 2023: 14 · 2022: 16 · 2021: 15 · 2020: 10 · 2019: 11 · 2018: 16 · 2017: 9 · 2016: 5 · 2015: 2
FWCI
6.84
Type
journal article
Language
en
Open access
closed
Locations
  • ACS Macro Letters (publishedVersion)
  • PubMed (publishedVersion)
  • HAL (submittedVersion)
Funders
Institut Universitaire de France
Topics
  • Physical Sciences › Materials Science › Polymers and Plastics › Polymer crystallization and properties
  • Physical Sciences › Materials Science › Materials Chemistry › Material Dynamics and Properties
  • Physical Sciences › Materials Science › Metals and Alloys › Microstructure and mechanical properties
Keywords
plastic deformation, semicrystalline polymers, amorphous polymers, strain softening, strain hardening, recrystallization, chain orientation, glass transition temperature, tensile properties

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