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Molecular Plasmonics with Tunable Exciton−Plasmon Coupling Strength in J-Aggregate Hybridized Au Nanorod Assemblies
Abstract
Controlling coherent electromagnetic interactions in molecular systems is a problem of both fundamental interest and important applicative potential in the development of photonic and opto-electronic devices. The strength of these interactions determines both the absorption and emission properties of molecules coupled to nanostructures, effectively governing the optical properties of such a composite metamaterial. Here we report on the observation of strong coupling between a plasmon supported by an assembly of oriented gold nanorods (ANR) and a molecular exciton. We show that the coupling is easily engineered and is deterministic as both spatial and spectral overlap between the plasmonic structure and molecular aggregates are controlled. We think that these results in conjunction with the flexible geometry of the ANR are of potential significance to the development of plasmonic molecular devices.
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Cites
Optical Constants of the Noble Metals
Johnson, P. B., & Christy, R. W. (1972) · Physical Review B · doi:10.1103/physrevb.6.4370 · Cited by 20,094
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Kabashin, A. V., Evans, P., Pastkovsky, S., Hendren, W., Wurtz, G. A., Atkinson, R., Pollard, R., Podolskiy, V. A., & Zayats, A. V. (2009) · Nature Materials · doi:10.1038/nmat2546 · Cited by 1,744
Self-citationStrong coupling between surface plasmon polaritons and emitters: a review
Törmä, P., & Barnes, W. L. (2015) · Reports on Progress in Physics · doi:10.1088/0034-4885/78/1/013901 · Cited by 1,644
Near-Field Mediated Plexcitonic Coupling and Giant Rabi Splitting in Individual Metallic Dimers
Schlather, A. E., Large, N., Urban, A. S., Nordlander, P., & Halas, N. J. (2013) · Nano Letters · doi:10.1021/nl4014887 · Cited by 537
Novel Nanostructures and Materials for Strong Light–Matter Interactions
Baranov, D. G., Wersäll, M., Cuadra, J., Antosiewicz, T. J., & Shegai, T. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b00674 · Cited by 531
Approaching the strong coupling limit in single plasmonic nanorods interacting with J-aggregates
Zengin, G., Johansson, G., Johansson, P., Antosiewicz, T. J., Käll, M., & Shegai, T. (2013) · Scientific Reports · doi:10.1038/srep03074 · Cited by 268
Metadata
- Authors
- Wurtz, G. A., Evans, P. R., Hendren, W., Atkinson, R., Dickson, W., Pollard, R. J., Zayats, A. V., Harrison, W., & Bower, C.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-04-25
- Volume
- 7
- Issue
- 5
- Pages
- 1297-1303
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2050680590
- Cited by
- 336
- References
- 1
- FWCI
- 11.43
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Wurtz, G. A., Evans, P. R., Hendren, W., Atkinson, R., Dickson, W., Pollard, R. J., Zayats, A. V., Harrison, W., & Bower, C. (2007). Molecular Plasmonics with Tunable Exciton−Plasmon Coupling Strength in J-Aggregate Hybridized Au Nanorod Assemblies. Nano Letters. https://doi.org/10.1021/nl070284m
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