The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Properties of Fluorinated Graphene Films
Abstract
Graphene films grown on Cu foils have been fluorinated with xenon difluoride (XeF(2)) gas on one or both sides. When exposed on one side the F coverage saturates at 25% (C(4)F), which is optically transparent, over 6 orders of magnitude more resistive than graphene, and readily patterned. Density functional calculations for varying coverages indicate that a C(4)F configuration is lowest in energy and that the calculated band gap increases with increasing coverage, becoming 2.93 eV for one C(4)F configuration. During defluorination, we find hydrazine treatment effectively removes fluorine while retaining graphene's carbon skeleton. The same films may be fluorinated on both sides by transferring graphene to a silicon-on-insulator substrate enabling XeF(2) gas to etch the Si underlayer and fluorinate the backside of the graphene film to form perfluorographane (CF) for which calculated the band gap is 3.07 eV. Our results indicate single-side fluorination provides the necessary electronic and optical changes to be practical for graphene device applications.
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Cites
Electric Field Effect in Atomically Thin Carbon Films
Novoselov, K. S., Geim, A. K., Morozov, S. V., Jiang, D., Zhang, Y., Dubonos, S. V., Grigorieva, I. V., & Firsov, A. A. (2004) · Science · doi:10.1126/science.1102896 · Cited by 66,834
Geim, A. K., & Novoselov, K. S. (2007) · Nature Materials · doi:10.1038/nmat1849 · Cited by 39,979
The electronic properties of graphene
Castro Neto, A. H., Guinea, F., Peres, N. M. R., Novoselov, K. S., & Geim, A. K. (2009) · Reviews of Modern Physics · doi:10.1103/revmodphys.81.109 · Cited by 24,803
Cited by
Dong, G., Zhang, Y., Pan, Q., & Qiu, J. (2014) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2014.04.002 · Cited by 1,085
First-principles investigation of graphene fluoride and graphane
Leenaerts, O., Peelaers, H., Hernández-Nieves, A. D., Partoens, B., & Peeters, F. M. (2010) · Physical Review B · doi:10.1103/physrevb.82.195436 · Cited by 462
Tribology of two-dimensional materials: From mechanisms to modulating strategies
Zhang, S., Ma, T., Erdemir, A., & Li, Q. (2019) · Materials Today · doi:10.1016/j.mattod.2018.12.002 · Cited by 407
How Do the Electrical Properties of Graphene Change with its Functionalization?
Sreeprasad, T. S., & Berry, V. (2013) · Small · doi:10.1002/smll.201202196 · Cited by 386
Chemistry Makes Graphene beyond Graphene
Liao, L., Peng, H., & Liu, Z. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5048297 · Cited by 319
Metadata
- Authors
- Robinson, J. T., Burgess, J. S., Junkermeier, C. E., Badescu, S. C., Reinecke, T. L., Perkins, F. K., Zalalutdniov, M. K., Baldwin, J. W., Culbertson, J. C., Sheehan, P. E., & Snow, E. S.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-07-16
- Volume
- 10
- Issue
- 8
- Pages
- 3001-3005
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W1993017167
- Cited by
- 1,131
- References
- 3
- FWCI
- 39.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Robinson, J. T., Burgess, J. S., Junkermeier, C. E., Badescu, S. C., Reinecke, T. L., Perkins, F. K., Zalalutdniov, M. K., Baldwin, J. W., Culbertson, J. C., Sheehan, P. E., & Snow, E. S. (2010). Properties of Fluorinated Graphene Films. Nano Letters. https://doi.org/10.1021/nl101437p
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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