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Cited by 304

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Purely Coherent Nonlinear Optical Response in Solution Dispersions of Graphene Sheets

Wu, Rui, Zhang, Yingli, Yan, Shichao, Bian, Fei, Wang, Wenlong, Bai, Xuedong, Lu, Xinghua, Zhao, Jimin, Wang, Enge·2011·Nano Letters

Abstract

We have developed an efficient chemical exfoliation approach for the high-throughput synthesis of solution-processable, high-quality graphene sheets that are noncovalently functionalized by alkylamine. Purely coherent nonlinear optical response of these graphene sheets has been investigated, using near-infrared, visible, and ultraviolet continous wave and ultrafast laser beams. Spatial self-phase modulation has been unambiguously observed in the solution dispersions. Our results suggest that this coherent light scattering is due to a broadband, ultrafast, and remarkably huge third-order optical nonlinearity χ(3), which is a manifestation of the graphene's cone-shaped large-energy-scale band structure. Our experimental findings endow graphene new potentials in nonlinear optical applications.

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Metadata

Authors
Wu, R., Zhang, Y., Yan, S., Bian, F., Wang, W., Bai, X., Lu, X., Zhao, J., & Wang, E.
Venue
Nano Letters
Published
2011-11-28
Volume
11
Issue
12
Pages
5159-5164
ISSN
  • 1530-6984 (ISSN-L)
  • 1530-6992
OpenAlex
W2091456106
Cited by
304
References
1
FWCI
3.87
Type
journal article
Language
en
Open access
closed

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