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Selective-Area Fluorination of Graphene with Fluoropolymer and Laser Irradiation
Abstract
We have devised a method to selectively fluorinate graphene by irradiating fluoropolymer-covered graphene with a laser. This fluoropolymer produces active fluorine radicals under laser irradiation that react with graphene but only in the laser-irradiated region. The kinetics of C-F bond formation is dependent on both the laser power and fluoropolymer thickness, proving that fluorination occurs by the decomposition of the fluoropolymer. Fluorination leads to a dramatic increase in the resistance of the graphene while the basic skeletal structure of the carbon bonding network is maintained. Considering the simplicity of the fluorination process and that it allows patterning with a nontoxic fluoropolymer as a solid source, this method could find application to generate fluorinated graphene in graphene-based electronic devices such as for the electrical isolation of graphene.
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Citations
Cites
Graphene: Status and Prospects
Geim, A. K. (2009) · Science · doi:10.1126/science.1158877 · Cited by 13,942
Thermal properties of graphene and nanostructured carbon materials
Balandin, A. A. (2011) · Nature Materials · doi:10.1038/nmat3064 · Cited by 6,244
Cited by
Chemistry Makes Graphene beyond Graphene
Liao, L., Peng, H., & Liu, Z. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5048297 · Cited by 319
Fluoropolymers in Biomedical Applications: State-of-the-Art and Future Perspectives
Lv, J., & Cheng, Y. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00258e · Cited by 316
Metadata
- Authors
- Lee, W. H., Suk, J. W., Chou, H., Lee, J., Hao, Y., Wu, Y., Piner, R., Akinwande, D., Kim, K. S., & Ruoff, R. S.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-04-06
- Volume
- 12
- Issue
- 5
- Pages
- 2374-2378
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2324824790
- Cited by
- 252
- References
- 2
- FWCI
- 13.90
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lee, W. H., Suk, J. W., Chou, H., Lee, J., Hao, Y., Wu, Y., Piner, R., Akinwande, D., Kim, K. S., & Ruoff, R. S. (2012). Selective-Area Fluorination of Graphene with Fluoropolymer and Laser Irradiation. Nano Letters. https://doi.org/10.1021/nl300346j
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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