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Direct Observation of Inhomogeneous Solid Electrolyte Interphase on MnO Anode with Atomic Force Microscopy and Spectroscopy
Abstract
Solid electrolyte interphase (SEI) is an in situ formed thin coating on lithium ion battery (LIB) electrodes. The mechanical property of SEI largely defines the cycling performance and the safety of LIBs but has been rarely investigated. Here, we report quantitatively the Young's modulus of SEI films on MnO anodes. The inhomogeneity of SEI film in morphology, structure, and mechanical properties provides new insights to the evolution of SEI on electrodes. Furthermore, the quantitative methodology established in this study opens a new approach to direct investigation of SEI properties in various electrode materials systems.
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Citations
Cited by
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Sodium Metal Anodes: Emerging Solutions to Dendrite Growth
Lee, B., Paek, E., Mitlin, D., & Lee, S. W. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00642 · Cited by 940
Emerging Era of Electrolyte Solvation Structure and Interfacial Model in Batteries
Cheng, H., Sun, Q., Li, L., Zou, Y., Wang, Y., Cai, T., Zhao, F., Liu, G., Ma, Z., Wahyudi, W., et al. (2022) · ACS Energy Letters · doi:10.1021/acsenergylett.1c02425 · Cited by 640
Exploring Anomalous Charge Storage in Anode Materials for Next-Generation Li Rechargeable Batteries
Kim, H., Choi, W., Yoon, J., Um, J. H., Lee, W., Kim, J., Cabana, J., & Yoon, W.-S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00618 · Cited by 527
Conversion Reaction‐Based Oxide Nanomaterials for Lithium Ion Battery Anodes
Yu, S., Lee, S. H., Lee, D. J., Sung, Y., & Hyeon, T. (2016) · Small · doi:10.1002/smll.201502299 · Cited by 499
Metadata
- Authors
- Zhang, J., Wang, R., Yang, X., Lu, W., Wu, X., Wang, X., Li, H., & Chen, L.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-03-09
- Volume
- 12
- Issue
- 4
- Pages
- 2153-2157
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2146566905
- Cited by
- 207
- References
- 0
- FWCI
- 7.33
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Zhang, J., Wang, R., Yang, X., Lu, W., Wu, X., Wang, X., Li, H., & Chen, L. (2012). Direct Observation of Inhomogeneous Solid Electrolyte Interphase on MnO Anode with Atomic Force Microscopy and Spectroscopy. Nano Letters. https://doi.org/10.1021/nl300570d
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