The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
Near-Field Mediated Plexcitonic Coupling and Giant Rabi Splitting in Individual Metallic Dimers
Abstract
Strong coupling between resonantly matched localized surface plasmons and molecular excitons results in the formation of new hybridized energy states called plexcitons. Understanding the nature and tunability of these hybrid nanostructures is important for both fundamental studies and the development of new applications. We investigate the interactions between J-aggregate excitons and single plasmonic dimers and report for the first time a unique strong coupling regime in individual plexcitonic nanostructures. Dark-field scattering measurements and finite-difference time-domain simulations of the hybrid nanostructures show strong plexcitonic coupling mediated by the near-field inside each dimer gap, which can be actively controlled by rotating the polarization of the optical excitation. The plexciton dispersion curves, obtained from coupled harmonic oscillator models, show anticrossing behavior at the exciton transition energy and giant Rabi splitting ranging between 230 and 400 meV. These energies are, to the best of our knowledge, the largest obtained on individual hybrid nanostructures.
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Cites
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Self-citationExciton−Plasmon Interaction and Hybrid Excitons in Semiconductor−Metal Nanoparticle Assemblies
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Surface plasmon resonance in gold nanoparticles: a review
Amendola, V., Pilot, R., Frasconi, M., Maragò, O. M., & Iatì, M. A. (2017) · Journal of Physics: Condensed Matter · doi:10.1088/1361-648x/aa60f3 · Cited by 1,905
Strong coupling between surface plasmon polaritons and emitters: a review
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Vacuum Rabi splitting in a plasmonic cavity at the single quantum emitter limit
Santhosh, K., Bitton, O., Chuntonov, L., & Haran, G. (2016) · Nature Communications · doi:10.1038/ncomms11823 · Cited by 675
Zengin, G., Wersäll, M., Nilsson, S., Antosiewicz, T. J., Käll, M., & Shegai, T. (2015) · Physical Review Letters · doi:10.1103/physrevlett.114.157401 · Cited by 566
Plasmon-Induced Hot Electron Transfer from the Au Tip to CdS Rod in CdS-Au Nanoheterostructures
Wu, K., Rodríguez-Córdoba, W. E., Yang, Y., & Lian, T. (2013) · Nano Letters · doi:10.1021/nl402730m · Cited by 334
Strong Light-Matter Interactions in Single Open Plasmonic Nanocavities at the Quantum Optics Limit
Liu, R., Zhou, Z.-K., Yu, Y.-C., Zhang, T., Wang, H., Liu, G., Wei, Y., Chen, H., & Wang, X.-H. (2017) · Physical Review Letters · doi:10.1103/physrevlett.118.237401 · Cited by 293
Approaching the strong coupling limit in single plasmonic nanorods interacting with J-aggregates
Zengin, G., Johansson, G., Johansson, P., Antosiewicz, T. J., Käll, M., & Shegai, T. (2013) · Scientific Reports · doi:10.1038/srep03074 · Cited by 268
Metadata
- Authors
- Schlather, A. E., Large, N., Urban, A. S., Nordlander, P., & Halas, N. J.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-06-13
- Volume
- 13
- Issue
- 7
- Pages
- 3281-3286
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2323117485
- Cited by
- 537
- References
- 31
- FWCI
- 23.91
- Type
- journal article
- Language
- en
- Open access
- closed
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