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Prelithiation of Silicon–Carbon Nanotube Anodes for Lithium Ion Batteries by Stabilized Lithium Metal Powder (SLMP)
Abstract
Stabilized lithium metal powder (SLMP) has been applied during battery assembly to effectively prelithiate high capacity (1500-2500 mAh/g) silicon-carbon nanotube (Si-CNT) anodes, eliminating the 20-40% first cycle irreversible capacity loss. Pressure-activation of SLMP is shown to enhance prelithiation and enable capacity matching between Si-CNT anodes and lithium nickel cobalt aluminum oxide (NCA) cathodes in full batteries with minimal added mass. The prelithiation approach enables high energy density NCA/Si-CNT batteries achieving >1000 cycles at 20% depth-of-discharge.
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Citations
Cited by
Hard Carbon as Sodium‐Ion Battery Anodes: Progress and Challenges
Xiao, B., Rojo, T., & Li, X. (2019) · ChemSusChem · doi:10.1002/cssc.201801879 · Cited by 432
Zhao, J., Lu, Z., Wang, H., Liu, W., Lee, H.-W., Yan, K., Zhuo, D., Lin, D., Liu, N., & Cui, Y. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b04526 · Cited by 369
Holtstiege, F., Bärmann, P., Nölle, R., Winter, M., & Placke, T. (2018) · Batteries · doi:10.3390/batteries4010004 · Cited by 357
High energy density calendered Si alloy/graphite anodes
Du, Z., Dunlap, R. A., & Obrovac, M. N. (2014) · Journal of The Electrochemical Society · doi:10.1149/2.0941410jes · Cited by 107
Metadata
- Authors
- Forney, M. W., Ganter, M. J., Staub, J. W., Ridgley, R. D., & Landi, B. J.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-08-08
- Volume
- 13
- Issue
- 9
- Pages
- 4158-4163
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2049938203
- Cited by
- 381
- References
- 0
- FWCI
- 12.38
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Prelithiation of Silicon–Carbon Nanotube Anodes for Lithium Ion Batteries by Stabilized Lithium Metal Powder (SLMP). https://app.cochat.ai/papers/10.1021/nl401776d
- The paper
- Forney, M. W., Ganter, M. J., Staub, J. W., Ridgley, R. D., & Landi, B. J. (2013). Prelithiation of Silicon–Carbon Nanotube Anodes for Lithium Ion Batteries by Stabilized Lithium Metal Powder (SLMP). Nano Letters. https://doi.org/10.1021/nl401776d
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Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
