The DOI matches its Crossref record; 25 of the 25 references it cites were found in a registry or an index.
Origin of Anomalous Water Permeation through Graphene Oxide Membrane
Open accessAbstract
Water inside the low-dimensional carbon structures has been considered seriously owing to fundamental interest in its flow and structures as well as its practical impact. Recently, the anomalous perfect penetration of water through graphene oxide membrane was demonstrated although the membrane was impenetrable for other liquids and even gases. The unusual auxetic behavior of graphene oxide in the presence of water was also reported. Here, on the basis of first-principles calculations, we establish atomistic models for hybrid systems composed of water and graphene oxides revealing the anomalous water behavior inside the stacked graphene oxides. We show that formation of hexagonal ice bilayer in between the flakes as well as melting transition of ice at the edges of flakes are crucial to realize the perfect water permeation across the whole stacked structures. The distance between adjacent layers that can be controlled either by oxygen reduction process or pressure is shown to determine the water flow thus highlighting a unique water dynamics in randomly connected two-dimensional spaces.
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Cites
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Cited by
Sun, P., Wang, K., & Zhu, H. (2016) · Advanced Materials · doi:10.1002/adma.201502595 · Cited by 668
High-Flux Graphene Oxide Nanofiltration Membrane Intercalated by Carbon Nanotubes
Han, Y., Jiang, Y., & Gao, C. (2015) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.5b00986 · Cited by 532
2D Laminar Membranes for Selective Water and Ion Transport
Kang, Y., Xia, Y., Wang, H., & Zhang, X. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201902014 · Cited by 325
Metadata
- Authors
- Boukhvalov, D. W., Katsnelson, M. I., & Son, Y.-W.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-07-19
- Volume
- 13
- Issue
- 8
- Pages
- 3930-3935
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2132036287
- Cited by
- 256
- References
- 25
- FWCI
- 12.05
- Type
- journal article
- Language
- en
- Open access
- green
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- Boukhvalov, D. W., Katsnelson, M. I., & Son, Y.-W. (2013). Origin of Anomalous Water Permeation through Graphene Oxide Membrane. Nano Letters. https://doi.org/10.1021/nl4020292
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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